Strain-regulated flexible molecular sensors enabled by 2D PtTe2

Zhehan Wang, Dingxuan Kang, Jiayi Chen, Xiao Xu, Xu Jing, Li Tao
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Abstract

Two-dimensional transition metal dichalcogenide (TMDs) holds great promise for future wearable technologies. The large-scale synthesis of TMDs and the investigation of their molecular sensing properties are current research hotspots. Herein, we construct flexible PtTe2 molecular sensors directly on polyimide, followed by the exploration on ammonia sensing properties and stability under strain. The sensor shows an excellent ammonia response of 0.4% ppm-1surpassing most reported semimetal-based sensors. In-situ sensing testing reveals 500% enhancement in response after controlled strain engineering, which suggests the potential to expand limit of detection and linearity range.
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二维PtTe2实现应变调节柔性分子传感器
二维过渡金属二硫化物(TMDs)在未来的可穿戴技术中具有很大的前景。大规模合成tmd及其分子传感性能的研究是当前的研究热点。本文直接在聚酰亚胺上构建柔性PtTe2分子传感器,并对其应变下的氨传感性能和稳定性进行了研究。该传感器表现出优异的氨响应0.4% ppm-1,超过了大多数报道的半金属基传感器。原位传感测试表明,控制应变工程后的响应提高了500%,这表明了扩大检测极限和线性范围的潜力。
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