Temperature and Excitation Dependence of Photoluminescence Spectra of InAs/GaAs Quantum Dot Heterostructures

T. Nee, Ya-Fen Wu, R. Lin, Jiunn-Chyi Lee
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Abstract

In this study we investigated the effects that the carrier dynamics have on the temperature- and excitation-intensity-dependent photoluminescence (PL) spectra of a self-assembled quantum dot heterostructure. A rate equation model is proposed to take into account the dot size distribution, the random population of density of states, state filling effects, and the important carrier transfer mechanisms for the quantum dot system, including carrier capture, relaxation, thermal emission, and retrapping. This model reproduces the PL spectra quite well. Our quantitative calculations of the behavior of the thermal emitting carriers under various incident power intensities within the temperature range 15−240 K explain the carrier transfer process quite reasonably for the quantum dot system. In addition, we discuss the thermal redistribution and state filling effects in detail in our analysis of the dependence of the PL spectra on the temperature and excitation power intensity applied to the sample.
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InAs/GaAs量子点异质结构光致发光光谱的温度和激发依赖性
在这项研究中,我们研究了载流子动力学对自组装量子点异质结构的温度和激发强度相关的光致发光(PL)光谱的影响。提出了考虑量子点系统中载流子捕获、弛豫、热发射和重陷等载流子转移机制的速率方程模型。该模型很好地再现了PL光谱。在15 ~ 240 K的温度范围内,我们对不同入射功率强度下的热发射载流子的行为进行了定量计算,相当合理地解释了量子点系统的载流子转移过程。此外,我们还详细讨论了热重分布和状态填充效应,并分析了样品的PL光谱与温度和激发功率强度的关系。
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