Numerical Reconstruction of Proton Exchange Membrane Fuel Cell Gas Diffusion Layers

Danan Yang, Himani Garg, Steven B. Beale, Martin Andersson
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Abstract

Stochastic reconstruction is widely employed for effective and flexible imitation of Gas Diffusion Layers (GDLs), e.g., to facilitate the study of their properties. However, the reconstruction often overlooks crucial factors such as fiber curvature, fiber stack arrangement, and fiber anisotropy. Consequently, the impact of these structural characteristics remains poorly understood. In this study, an in-house reconstruction procedure is developed based on the periodic surface model. This procedure enables the generation of GDLs with either straight or curved fibers, layer-by-layer or random arrangement, and different probabilities of through-plane fiber orientation angles. The porosity, domain size, and fiber diameter are extracted from an experimental image-based GDL and utilized as input data for the reconstruction. Furthermore, the different GDLs are compared in terms of pore size distribution and through-plane porosity distribution. It is concluded that introducing proper selections of these fiber features gives the reconstruction more realistic properties.
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质子交换膜燃料电池气体扩散层的数值重建
随机重建被广泛用于有效和灵活地模拟气体扩散层(gdl),例如便于研究其性质。然而,这种重构往往忽略了光纤曲率、光纤堆叠排列和光纤各向异性等关键因素。因此,这些结构特征的影响仍然知之甚少。在本研究中,开发了一种基于周期曲面模型的内部重建程序。该方法可以生成直线或弯曲光纤,分层或随机排列,以及不同概率的穿过平面的光纤取向角的gdl。从基于实验图像的GDL中提取孔隙度、区域尺寸和纤维直径,并将其作为重建的输入数据。此外,还比较了不同GDLs的孔径分布和通面孔隙度分布。通过对这些纤维特性的适当选择,可以使重建的材料具有更真实的性能。
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