Evaluation of CO2 Adsorption Parameters in Fluidised Zeolite 13X Beds Using Non-Linear Multivariate Optimisation

IF 2.5 4区 工程技术 Q3 CHEMISTRY, ANALYTICAL Separations Pub Date : 2023-11-03 DOI:10.3390/separations10110558
Alessio Caravella, Giuseppe Prenesti, Salvatore De Luca, Maria Turano, Flaviano Testa, Rossella Girimonte
{"title":"Evaluation of CO2 Adsorption Parameters in Fluidised Zeolite 13X Beds Using Non-Linear Multivariate Optimisation","authors":"Alessio Caravella, Giuseppe Prenesti, Salvatore De Luca, Maria Turano, Flaviano Testa, Rossella Girimonte","doi":"10.3390/separations10110558","DOIUrl":null,"url":null,"abstract":"This work is part of a research project aimed at studying potential sorbents for CO2 capture. The main parameters characterising the adsorption process of zeolite 13X were derived with the aim of overcoming the limits of experimental analysis and thus predicting the performances of the materials of interest. In particular, the main parameters that control the adsorption process of CO2 in zeolite 13X were evaluated through parametric optimisation. This systematic procedure allows for the prediction of the performances of the materials at different operating conditions, identifying the most suitable ones for the case under consideration. Another important application lies in the possibility of a preliminary study of a potential process scale-up for future industrial use. The captured carbon dioxide can be stored or used as a reagent in the production of products with higher economic values, such as methanol, DME and others.","PeriodicalId":21833,"journal":{"name":"Separations","volume":"35 11","pages":"0"},"PeriodicalIF":2.5000,"publicationDate":"2023-11-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Separations","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.3390/separations10110558","RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, ANALYTICAL","Score":null,"Total":0}
引用次数: 0

Abstract

This work is part of a research project aimed at studying potential sorbents for CO2 capture. The main parameters characterising the adsorption process of zeolite 13X were derived with the aim of overcoming the limits of experimental analysis and thus predicting the performances of the materials of interest. In particular, the main parameters that control the adsorption process of CO2 in zeolite 13X were evaluated through parametric optimisation. This systematic procedure allows for the prediction of the performances of the materials at different operating conditions, identifying the most suitable ones for the case under consideration. Another important application lies in the possibility of a preliminary study of a potential process scale-up for future industrial use. The captured carbon dioxide can be stored or used as a reagent in the production of products with higher economic values, such as methanol, DME and others.
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
用非线性多元优化评价沸石13X流化床CO2吸附参数
这项工作是一个研究项目的一部分,旨在研究二氧化碳捕获的潜在吸附剂。推导了表征沸石13X吸附过程的主要参数,目的是克服实验分析的局限性,从而预测感兴趣材料的性能。通过参数优化,对控制CO2在13X分子筛上吸附过程的主要参数进行了评价。该系统程序允许预测材料在不同操作条件下的性能,确定最适合所考虑的情况的材料。另一个重要的应用是对未来工业用途的潜在工艺放大进行初步研究的可能性。捕获的二氧化碳可以储存起来或用作生产具有较高经济价值的产品的试剂,如甲醇、二甲醚等。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 去求助
来源期刊
Separations
Separations Chemistry-Analytical Chemistry
CiteScore
3.00
自引率
15.40%
发文量
342
审稿时长
12 weeks
期刊介绍: Separations (formerly Chromatography, ISSN 2227-9075, CODEN: CHROBV) provides an advanced forum for separation and purification science and technology in all areas of chemical, biological and physical science. It publishes reviews, regular research papers and communications. Our aim is to encourage scientists to publish their experimental and theoretical results in as much detail as possible. There is no restriction on the length of the papers. The full experimental details must be provided so that the results can be reproduced. There are, in addition, unique features of this journal: Manuscripts regarding research proposals and research ideas will be particularly welcomed. Electronic files and software regarding the full details of the calculation and experimental procedure, if unable to be published in a normal way, can be deposited as supplementary material. Manuscripts concerning summaries and surveys on research cooperation and projects (that are funded by national governments) to give information for a broad field of users. The scope of the journal includes but is not limited to: Theory and methodology (theory of separation methods, sample preparation, instrumental and column developments, new separation methodologies, etc.) Equipment and techniques, novel hyphenated analytical solutions (significantly extended by their combination with spectroscopic methods and in particular, mass spectrometry) Novel analysis approaches and applications to solve analytical challenges which utilize chromatographic separations as a key step in the overall solution Computational modelling of separations for the purpose of fundamental understanding and/or chromatographic optimization
期刊最新文献
Effective Utilization of Sulfur Wastewater by Photocatalytic System Using B/CuO/ZnO A Cyanoalkyl Silicone GC Stationary-Phase Polymer as an Extractant for Dispersive Liquid–Liquid Microextraction Central European Group for Separation Sciences (CEGSS)—Brief History and Memoirs on the Creation and Activity Effect of Fly Ash on the Mass Transfer Performance of CO2 Removal Using MEA and DEA Solutions in a Packed Tower Adsorption Performance and Mechanism of H3PO4-Modified Banana Peel Hydrothermal Carbon on Pb(II)
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1