A novel flow electrode capacitive deionization device with spindle-shaped desalting chamber

IF 6.1 2区 环境科学与生态学 Q2 ENGINEERING, ENVIRONMENTAL Frontiers of Environmental Science & Engineering Pub Date : 2023-12-10 DOI:10.1007/s11783-024-1800-y
Yunke Li, Junjun Ma, Chenxu Yang, Jianrui Niu, Yonghuan Bian, Ruicheng Chen, Puming Zhang, Jing Zhang, Chun Liu
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Abstract

Flow-electrode capacitive deionization (FCDI) is an innovative technology in which an intermediate chamber plays an important role in the desalination process. However, relatively few studies have been conducted on the structures of these intermediate chambers. In this study, we propose a novel flow-electrode capacitive deionization device with a spindle-shaped inlet chamber (S-FCDI). The desalination rate of the S-FCDI under optimal operating conditions was 36% higher than that of the FCDI device with a conventional rectangular chamber (R-FCDI). The spindle-shaped chamber transferred 1.2 µmol more ions than the rectangular chamber, based on energy per joule. Additionally, we performed a detailed analysis of different inlet chamber shapes using computational fluid dynamics software. We concluded that S-FCDI has a relatively low flow resistance and almost no stagnation zone. This provides unique insights into the development of intermediate chambers. This study may contribute to the improvement of the desalination performance in industrial applications of FCDI.

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带纺锤形脱盐室的新型流动电极电容式去离子装置
流电极电容式去离子(FCDI)是一种创新技术,其中中间室在海水淡化过程中发挥着重要作用。然而,有关这些中间室结构的研究相对较少。在本研究中,我们提出了一种具有纺锤形进水室的新型流电极电容式去离子装置(S-FCDI)。在最佳运行条件下,S-FCDI 的脱盐率比带有传统矩形腔体的 FCDI 设备(R-FCDI)高 36%。按每焦耳能量计算,纺锤形腔体比矩形腔体多传输 1.2 µmol 的离子。此外,我们还使用计算流体动力学软件对不同形状的入口室进行了详细分析。我们得出结论,S-FCDI 的流动阻力相对较小,几乎没有停滞区。这为中间腔的开发提供了独特的见解。这项研究可能有助于提高 FCDI 工业应用中的脱盐性能。
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来源期刊
Frontiers of Environmental Science & Engineering
Frontiers of Environmental Science & Engineering ENGINEERING, ENVIRONMENTAL-ENVIRONMENTAL SCIENCES
CiteScore
10.90
自引率
12.50%
发文量
988
审稿时长
6.1 months
期刊介绍: Frontiers of Environmental Science & Engineering (FESE) is an international journal for researchers interested in a wide range of environmental disciplines. The journal''s aim is to advance and disseminate knowledge in all main branches of environmental science & engineering. The journal emphasizes papers in developing fields, as well as papers showing the interaction between environmental disciplines and other disciplines. FESE is a bi-monthly journal. Its peer-reviewed contents consist of a broad blend of reviews, research papers, policy analyses, short communications, and opinions. Nonscheduled “special issue” and "hot topic", including a review article followed by a couple of related research articles, are organized to publish novel contributions and breaking results on all aspects of environmental field.
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