Triboelectric power generation performance of polyvinyl alcohol using ZnO–CuO–AgO trimetallic nanoparticles

IF 3.6 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Materials for Renewable and Sustainable Energy Pub Date : 2024-05-21 DOI:10.1007/s40243-024-00264-9
Swathi Yempally, Sumalatha Bonthula, Deepalekshmi Ponnamma
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Abstract

Triboelectric nanogenerators (TENGs), a new technology for gathering sustainable energy, have attracted much scientific interest. In this study, we describe a unique method for modifying the triboelectric power generation performance of Polyvinyl Alcohol (PVA) by adding ZnO–CuO–AgO (ZCA) trimetallic nanoparticles to improve the performance of TENGs and answer the requirement for ecologically benign and biodegradable materials. Hydrothermal synthesis adopted to create ZnO–CuO–AgO trimetallic nanoparticles ensures a distinctive structure with a large surface area, essential for enhancing triboelectric power generation. From the AFM results, it is evident that 1% PVA/ZCA showed the highest output voltage of 0.27V. Despite following the general trend, at higher concentrations of ZCA nanofiller in the PVA matrix, the enhancement of output voltage is not observed, which can be attributed to the non-uniform distribution. The effect of spin-coated film thickness and nanoparticle concentration on the triboelectric performance of the PVA nanogenerator is studied by monitoring the open-circuit voltage in response to various mechanical stimuli. Finally, the developed biodegradable nanogenerators in this study can be used for sustainable energy harvesting applications such as wearable electronics, self-powered sensors, and environmental monitoring systems.

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使用 ZnO-CuO-AgO 三金属纳米粒子的聚乙烯醇三电发电性能
三电纳米发电机(TENGs)作为一种收集可持续能源的新技术,已经引起了科学界的广泛关注。在本研究中,我们介绍了一种独特的方法,通过添加 ZnO-CuO-AgO (ZCA)三金属纳米粒子来改变聚乙烯醇(PVA)的三电发电性能,从而提高 TENG 的性能,满足对生态良性和可生物降解材料的要求。采用水热合成法制造的 ZnO-CuO-AgO 三金属纳米粒子具有独特的结构和较大的比表面积,对提高三电发电性能至关重要。从原子力显微镜结果可以看出,1% PVA/ZCA 的输出电压最高,为 0.27V。尽管遵循了一般趋势,但当 PVA 基体中的 ZCA 纳米填料浓度较高时,输出电压并没有增强,这可能是由于分布不均匀造成的。通过监测开路电压对各种机械刺激的响应,研究了旋涂薄膜厚度和纳米粒子浓度对 PVA 纳米发电机三电性能的影响。最后,本研究开发的可生物降解纳米发电机可用于可持续能源采集应用,如可穿戴电子设备、自供电传感器和环境监测系统。
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来源期刊
Materials for Renewable and Sustainable Energy
Materials for Renewable and Sustainable Energy MATERIALS SCIENCE, MULTIDISCIPLINARY-
CiteScore
7.90
自引率
2.20%
发文量
8
审稿时长
13 weeks
期刊介绍: Energy is the single most valuable resource for human activity and the basis for all human progress. Materials play a key role in enabling technologies that can offer promising solutions to achieve renewable and sustainable energy pathways for the future. Materials for Renewable and Sustainable Energy has been established to be the world''s foremost interdisciplinary forum for publication of research on all aspects of the study of materials for the deployment of renewable and sustainable energy technologies. The journal covers experimental and theoretical aspects of materials and prototype devices for sustainable energy conversion, storage, and saving, together with materials needed for renewable fuel production. It publishes reviews, original research articles, rapid communications, and perspectives. All manuscripts are peer-reviewed for scientific quality. Topics include: 1. MATERIALS for renewable energy storage and conversion: Batteries, Supercapacitors, Fuel cells, Hydrogen storage, and Photovoltaics and solar cells. 2. MATERIALS for renewable and sustainable fuel production: Hydrogen production and fuel generation from renewables (catalysis), Solar-driven reactions to hydrogen and fuels from renewables (photocatalysis), Biofuels, and Carbon dioxide sequestration and conversion. 3. MATERIALS for energy saving: Thermoelectrics, Novel illumination sources for efficient lighting, and Energy saving in buildings. 4. MATERIALS modeling and theoretical aspects. 5. Advanced characterization techniques of MATERIALS Materials for Renewable and Sustainable Energy is committed to upholding the integrity of the scientific record. As a member of the Committee on Publication Ethics (COPE) the journal will follow the COPE guidelines on how to deal with potential acts of misconduct. Authors should refrain from misrepresenting research results which could damage the trust in the journal and ultimately the entire scientific endeavor. Maintaining integrity of the research and its presentation can be achieved by following the rules of good scientific practice as detailed here: https://www.springer.com/us/editorial-policies
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