First-principles and experimental insight of high-entropy materials as electrocatalysts for energy-related applications: Hydrogen evolution, oxygen evolution, and oxygen reduction reactions

IF 31.6 1区材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Materials Science and Engineering: R: Reports Pub Date : 2024-06-27 DOI:10.1016/j.mser.2024.100813

Jasmin S. Shaikh , Meena Rittiruam , Tinnakorn Saelee , Victor Márquez , Navajsharif S. Shaikh , Patcharaporn Khajondetchairit , Sumayya Pathan , Pongsakorn Kanjanaboos , Toshiaki Taniike , Mohammad Khaja Nazeeruddin , Piyasan Praserthdam , Supareak Praserthdam

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Abstract

High entropy materials (HEMs) are highly effective as a catalyst and can be synthesized by facile methods. Here, we discuss recent advancements in HEMs for Hydrogen evolution reaction (HER), Oxygen evolution reaction (OER), and Oxygen reduction reaction (ORR) via electrocatalysis. We introduce newly emerged HEMs in different aspects: advanced synthesis, characterization techniques, and computational tools for analysis relating to the surface, lattice, defect, and interface. Additionally, this review provides detailed information on HEMs and their properties. It also explores rational approaches in the design of emerging HEMs based on first-principles calculations.

HEMs have potential roles as a catalyst in the field of energy production, energy conversion, and energy storage. The properties of HEMs can be enhanced through the integration of various functional materials, aiming for high resilience and excellent efficacy. In this review, we discussed synthesis of HEMs and their roles in the field of electrocatalysis considering theoretical, experimental, and pragmatic approaches.

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高熵材料作为能源相关应用电催化剂的第一原理和实验见解：氢进化、氧进化和氧还原反应

高熵材料 (HEM) 作为催化剂非常有效，而且可以通过简便的方法合成。在此，我们将讨论通过电催化实现氢进化反应（HER）、氧进化反应（OER）和氧还原反应（ORR）的高熵材料的最新进展。我们从不同方面介绍了新出现的 HEM：先进的合成、表征技术以及用于分析表面、晶格、缺陷和界面的计算工具。此外，本综述还提供了有关 HEMs 及其特性的详细信息。HEMs 在能源生产、能源转换和能源存储领域具有潜在的催化剂作用。HEMs 在能源生产、能源转换和能源存储领域具有潜在的催化剂作用。通过整合各种功能材料，可以增强 HEMs 的性能，从而实现高弹性和卓越功效。在这篇综述中，我们从理论、实验和实际操作等方面探讨了 HEMs 的合成及其在电催化领域的作用。

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来源期刊

Materials Science and Engineering: R: Reports 工程技术-材料科学：综合

CiteScore

60.50

自引率

0.30%

发文量

审稿时长

34 days

期刊介绍： Materials Science & Engineering R: Reports is a journal that covers a wide range of topics in the field of materials science and engineering. It publishes both experimental and theoretical research papers, providing background information and critical assessments on various topics. The journal aims to publish high-quality and novel research papers and reviews. The subject areas covered by the journal include Materials Science (General), Electronic Materials, Optical Materials, and Magnetic Materials. In addition to regular issues, the journal also publishes special issues on key themes in the field of materials science, including Energy Materials, Materials for Health, Materials Discovery, Innovation for High Value Manufacturing, and Sustainable Materials development.