A high-entropy strategy for stable structure of sodium ion batteries: From fundamentals to applications

IF 13.3 1区 工程技术 Q1 ENGINEERING, CHEMICAL Chemical Engineering Journal Pub Date : 2024-07-05 DOI:10.1016/j.cej.2024.153743
Xu Liu , Xin-Yu Liu , Nan Zhang , Peng-Fei Wang , Zong-Lin Liu , Jun-Hong Zhang , Jie Shu , Yan Sun , Chun-Sheng Li , Ting-Feng Yi
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Abstract

Sodium-ion batteries are excellent candidates for next-generation large-scale energy storage, but their performance is not yet comparable to high-level rechargeable batteries. Therefore, the development of Na-storage materials with excellent performance is crucial. Recently, high-entropy materials have gained attention due to their multi-component synergistic effect and adjustable energy storage characteristics. This is expected to overcome the comprehensive performance bottleneck of traditional materials, providing new opportunities for accelerating the development of Na-storage materials. This review summarizes the latest research results of high-entropy strategy in the field of sodium-ion batteries, including cathode, anode, and solid electrolyte. The review provides an in-depth understanding of the structural changes and performance advantages of high-entropy materials and provides a detailed introduction to the key role of high-entropy strategy in maintaining structural stability, suppressing irreversible phase transitions, and improving ion transport. Finally, we present several understandings of the future challenges and opportunities that high-entropy Na-storage materials. Some enlightening guidance is provided for further research on high-entropy substitution strategy for Na-storage materials.

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钠离子电池稳定结构的高熵策略:从基础到应用
钠离子电池是下一代大规模储能的绝佳候选材料,但其性能还无法与高级充电电池相媲美。因此,开发性能优异的钠离子储能材料至关重要。最近,高熵材料因其多组分协同效应和可调节的储能特性而备受关注。这有望突破传统材料的综合性能瓶颈,为加快储纳材料的发展提供新的机遇。本综述总结了高熵策略在钠离子电池领域的最新研究成果,包括正极、负极和固体电解质。综述深入介绍了高熵材料的结构变化和性能优势,并详细介绍了高熵策略在保持结构稳定、抑制不可逆相变和改善离子传输方面的关键作用。最后,我们介绍了对高熵贮钠材料未来挑战和机遇的几点理解。为进一步研究贮钠材料的高熵替代策略提供了一些启发性指导。
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来源期刊
Chemical Engineering Journal
Chemical Engineering Journal 工程技术-工程:化工
CiteScore
21.70
自引率
9.30%
发文量
6781
审稿时长
2.4 months
期刊介绍: The Chemical Engineering Journal is an international research journal that invites contributions of original and novel fundamental research. It aims to provide an international platform for presenting original fundamental research, interpretative reviews, and discussions on new developments in chemical engineering. The journal welcomes papers that describe novel theory and its practical application, as well as those that demonstrate the transfer of techniques from other disciplines. It also welcomes reports on carefully conducted experimental work that is soundly interpreted. The main focus of the journal is on original and rigorous research results that have broad significance. The Catalysis section within the Chemical Engineering Journal focuses specifically on Experimental and Theoretical studies in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. These studies have industrial impact on various sectors such as chemicals, energy, materials, foods, healthcare, and environmental protection.
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