Investigations on conical lean turbulent premixed hydrogenated natural gas flames

Dilay Güleryüz , Christophe Allouis , İskender Gökalp
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Abstract

Hydrogen's ability to enhance carbon neutrality in combustion processes puts forward the use of hydrogenated fuels, both in the form of fuel and an energy carrier as a potential decarbonization solution. However, because of the nature of hydrogen, blending it with hydrocarbons causes crucial structural changes in the flame structure, including higher flame propagation velocities and higher flame temperatures, decreased instantaneous flame thickness, and increased risks of flame flashback and an increasing potential of NOx emissions due to higher flame temperatures. These attributes encourage a thorough examination of hydrogenated blends of hydrocarbon fuels. Using lean premixed fuels is another technique to achieve efficient and cleaner combustion. However, due to the problem of flame instability in lean premixed combustion, forecasting the design points in terms of flame attributes is critical for better combustor designs.

In this study, conical (Bunsen type) lean premixed turbulent flames of hydrogenated natural gas-air mixtures are experimentally studied. Through chemiluminescence measurements of the OH* and CH* radicals and laser-induced Mie scattering, lean natural gas-air premixed flames are examined with subsequently increasing hydrogen addition rates up to 20% by volume and keeping the premixture velocity constant. The obtained data is utilized for exploring the dynamics of the turbulent flame front. The main turbulent premixed flame parameters we identified relate to the instantaneous and average topology of the flame such as the turbulent flame brush thickness and flame height. We also inferred global combustion parameters like the turbulent flame propagation speed from the experimental findings.

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锥形贫化湍流预混合加氢天然气火焰研究
氢气能够提高燃烧过程中的碳中性,因此氢化燃料的使用,无论是作为燃料还是作为能源载体,都是一种潜在的脱碳解决方案。然而,由于氢的特性,氢与碳氢化合物混合会导致火焰结构发生重大变化,包括火焰传播速度加快、火焰温度升高、瞬时火焰厚度减小、火焰回火风险增加以及火焰温度升高导致氮氧化物排放潜力增加。这些特性促使我们对碳氢化合物燃料的加氢混合物进行彻底研究。使用贫油预混燃料是实现高效清洁燃烧的另一种技术。然而,由于贫油预混燃烧中的火焰不稳定性问题,预测火焰属性方面的设计点对于更好地设计燃烧器至关重要。本研究对加氢天然气-空气混合物的锥形(本生型)贫油预混湍流火焰进行了实验研究。通过对 OH* 和 CH* 自由基的化学发光测量以及激光诱导 Mie 散射,研究了在保持预混速度不变的情况下,随着氢气添加率的增加(按体积计算最高可达 20%),贫天然气-空气预混合火焰的情况。获得的数据用于探索湍流火焰前沿的动态。我们确定的主要湍流预混火焰参数与火焰的瞬时和平均拓扑结构有关,如湍流火焰刷厚度和火焰高度。我们还从实验结果中推断出了湍流火焰传播速度等全局燃烧参数。
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