PM2.5 estimated directly from satellite data and from fused data produced by an interpretable multi-model stacking ensemble method

IF 3.9 3区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES Atmospheric Pollution Research Pub Date : 2024-07-16 DOI:10.1016/j.apr.2024.102259
Xingxing Ma , Hongnian Liu , Qian Liu , Yuanmou Wang
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Abstract

Rapid urbanization and industrialization in China have resulted in an increase of PM2.5 concentrations. In this study, an interpretable multi-model stacking ensemble method (IMSEM) with top-of-the-atmosphere reflectance (TOAR) from the Himawari-8 satellite were used to acquire high-resolution PM2.5 data in China. In contrast to the traditional approach whereby PM2.5 is estimated with single models, using TOAR data, IMSEM outperformed single models in terms of several skill scores. The hourly average R2 (RMSE) of 10-fold-cross validation reached 0.84 (9.52 μg/m3) in 2021 by IMSEM. The feature importance results of IMSEM showed the significant contributions of TOAR and meteorological variables. The PM2.5 estimates of IMSEM were also fused with surface observations using interpolation for correction and optimization. When this was done for PM2.5 concentrations in 2022, it was found that, among the four seasons, the fusion-based estimate of PM2.5 concentration was highest in winter (49.94 μg/m3), followed by autumn (31.59 μg/m3) and spring (29.07 μg/m3), and lowest in summer (19.25 μg/m3).

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直接从卫星数据和可解释的多模型叠加集合方法产生的融合数据估算的 PM2.5
中国的快速城市化和工业化导致 PM2.5 浓度上升。本研究利用可解释的多模式叠加集合方法(IMSEM)和向日葵8号卫星的大气顶部反射率(TOAR)获取了中国的高分辨率PM2.5数据。与使用单一模型估算 PM2.5 的传统方法相比,利用 TOAR 数据,IMSEM 在多个技能评分方面均优于单一模型。在 2021 年,IMSEM 的 10 倍交叉验证的小时平均 R2(RMSE)达到 0.84(9.52 μg/m3)。IMSEM的特征重要性结果显示,TOAR和气象变量的贡献显著。IMSEM的PM2.5估计值还与地面观测数据融合,使用插值法进行校正和优化。在对2022年的PM2.5浓度进行融合时发现,在四个季节中,基于融合的PM2.5浓度估计值在冬季最高(49.94 μg/m3),其次是秋季(31.59 μg/m3)和春季(29.07 μg/m3),夏季最低(19.25 μg/m3)。
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来源期刊
Atmospheric Pollution Research
Atmospheric Pollution Research ENVIRONMENTAL SCIENCES-
CiteScore
8.30
自引率
6.70%
发文量
256
审稿时长
36 days
期刊介绍: Atmospheric Pollution Research (APR) is an international journal designed for the publication of articles on air pollution. Papers should present novel experimental results, theory and modeling of air pollution on local, regional, or global scales. Areas covered are research on inorganic, organic, and persistent organic air pollutants, air quality monitoring, air quality management, atmospheric dispersion and transport, air-surface (soil, water, and vegetation) exchange of pollutants, dry and wet deposition, indoor air quality, exposure assessment, health effects, satellite measurements, natural emissions, atmospheric chemistry, greenhouse gases, and effects on climate change.
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