Activation cross section for 85Rb(n,2n)84mRb and 85Rb(n,p)85mKr reactions with uncertainty propagation and covariance analysis

IF 1.5 3区 化学 Q3 CHEMISTRY, ANALYTICAL Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2024-09-05 DOI:10.1007/s10967-024-09682-5
Mayur Mehta, N. L. Singh, Ratankumar Singh, R. Makwana, P. V. Subhash, Rakesh Chauhan, S. V. Suryanarayana, K. Katovsky
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Abstract

The cross section of 85Rb(n,2n)84mRb and 85Rb(n,p)85mKr reactions were measured at neutron energy range 12–20 MeV using activation analysis followed by off-line γ-ray spectroscopic technique. The quasi mono-energetic neutrons were produced through 7Li(p,n)7Be reaction. The measurements were done relative to 27Al(n,α)24Na reference monitor reaction cross section. The detailed uncertainty propagation from the attributes present in measurements was performed using covariance analysis. The γ-ray self-attenuation and background low neutron energy corrections were performed in the measurement studies. Theoretical calculations were performed by TALYS-1.96 nuclear code. The comparison of measured values with the available data in EXFOR database and evaluated data from JENDL-5 and EAF-2010 shows the measured cross section values of 85Rb(n,p)85mKr reaction were slightly higher than the published values, evaluated data and theoretical data while for 85Rb(n,2n)84mRb, the measured values were consistent with the published data.

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带有不确定性传播和协方差分析的 85Rb(n,2n)84mRb 和 85Rb(n,p)85mKr 反应的活化截面
在中子能量范围为 12-20 MeV 时,利用活化分析和离线 γ 射线光谱技术测量了 85Rb(n,2n)84mRb 和 85Rb(n,p)85mKr 反应的截面。准单能中子是通过 7Li(p,n)7Be 反应产生的。测量是相对于 27Al(n,α)24Na参照监测器反应截面进行的。利用协方差分析对测量中存在的属性进行了详细的不确定性传播。在测量研究中进行了 γ 射线自衰减和背景低中子能量修正。理论计算由 TALYS-1.96 核代码完成。将测量值与 EXFOR 数据库中的现有数据以及 JENDL-5 和 EAF-2010 的评估数据进行比较后发现,85Rb(n,p)85mKr 反应的测量截面值略高于公布值、评估数据和理论数据,而对于 85Rb(n,2n)84mRb,测量值与公布数据一致。
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来源期刊
CiteScore
2.80
自引率
18.80%
发文量
504
审稿时长
2.2 months
期刊介绍: An international periodical publishing original papers, letters, review papers and short communications on nuclear chemistry. The subjects covered include: Nuclear chemistry, Radiochemistry, Radiation chemistry, Radiobiological chemistry, Environmental radiochemistry, Production and control of radioisotopes and labelled compounds, Nuclear power plant chemistry, Nuclear fuel chemistry, Radioanalytical chemistry, Radiation detection and measurement, Nuclear instrumentation and automation, etc.
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