Ti3C2Tx Aerogel-Based Wearable Humidity Sensors with Low Hysteresis and High Linearity for Expiratory Comfort Management

IF 9.1 1区 化学 Q1 CHEMISTRY, ANALYTICAL ACS Sensors Pub Date : 2024-11-26 DOI:10.1021/acssensors.4c02338
Yanan Xiao, Qi Pu, Xiaoteng Jia, Tianyi Gu, Yong Liu, Peng Sun, Fangmeng Liu, Geyu Lu
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Abstract

Wearable and flexible humidity sensors hold great promise for expiratory comfort management. However, the high hysteresis and poor detection linearity restrict the immediate and accurate detection of humidity. Herein, we have prepared Ti3C2Tx MXene/chitosan/polyvinylidene difluoride aerogels with a controllable hydrophobic/hydrophilic surface to regulate the catch/escape behavior of H2O molecules. The MXene aerogel-based humidity sensor demonstrates low hysteresis (3.2% relative humidity) and a high linear relationship (R2 = 0.99). Integrated with a control circuit, an expiratory humidity monitoring system is constructed for nasal comfort management as a humidity switch. The exhaled breath humidity can be automatically regulated during dry exhalation conditions. This wearable humidity sensor enables the real-time monitoring and intelligent control of nasal exhaled humidity. This work represents a new avenue for improving breathing comfort and preventing respiratory diseases.

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基于 Ti3C2Tx 气凝胶的可穿戴湿度传感器具有低滞后和高线性度,适用于呼气舒适度管理
可穿戴的柔性湿度传感器在呼气舒适度管理方面大有可为。然而,高滞后性和较差的检测线性限制了湿度的即时准确检测。在此,我们制备了具有可控疏水/亲水表面的 Ti3C2Tx MXene/壳聚糖/聚偏二氟乙烯气凝胶,以调节 H2O 分子的捕捉/逃逸行为。基于 MXene 气凝胶的湿度传感器具有较低的滞后(相对湿度为 3.2%)和较高的线性关系(R2 = 0.99)。通过与控制电路的集成,构建了一个呼气湿度监测系统,作为湿度开关用于鼻腔舒适度管理。在呼气干燥的情况下,呼气湿度可自动调节。这种可穿戴湿度传感器可实现对鼻腔呼气湿度的实时监测和智能控制。这项工作为改善呼吸舒适度和预防呼吸系统疾病开辟了一条新途径。
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来源期刊
ACS Sensors
ACS Sensors Chemical Engineering-Bioengineering
CiteScore
14.50
自引率
3.40%
发文量
372
期刊介绍: ACS Sensors is a peer-reviewed research journal that focuses on the dissemination of new and original knowledge in the field of sensor science, particularly those that selectively sense chemical or biological species or processes. The journal covers a broad range of topics, including but not limited to biosensors, chemical sensors, gas sensors, intracellular sensors, single molecule sensors, cell chips, and microfluidic devices. It aims to publish articles that address conceptual advances in sensing technology applicable to various types of analytes or application papers that report on the use of existing sensing concepts in new ways or for new analytes.
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