Metallic Electro-optic Effect in Gapped Bilayer Graphene

IF 9.6 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nano Letters Pub Date : 2025-01-15 DOI:10.1021/acs.nanolett.4c03771
Da Ma, Ying Xiong, Justin C. W. Song
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Abstract

Electro-optic (EO) modulation is a critical device action in photonics. Recently, the non-Drude dynamics induced by the Berry curvature dipole (BCD) in metals have attracted attention as a potential candidate for terahertz EO modulation. However, such BCD-induced EO effects can be challenging to realize, often requiring flat bands and complex materials such as a strained magic-angle twisted bilayer graphene on hexagonal boron nitride. Here, we argue that metallic EO can be achieved with a much simpler material, gapped bilayer graphene, with EO coefficients comparable to that in flat-band materials in the terahertz range. In particular, we find metallic EO can be realized without a Berry curvature dipole; we identify skew-scattering and a “snap” (third-order derivative of velocity) can readily produce pronounced Pockels and Kerr EO effects in clean metals. These yield nonreciprocal and field-activated birefringence and field-induced modulations to transmission and reflection, essential components for terahertz EO modulators.

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来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
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