Evidence of Heating-Dominated Urban NOx Emissions

IF 11.3 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL 环境科学与技术 Pub Date : 2025-02-28 DOI:10.1021/acs.est.4c13276
Samuel J. Cliff, Will Drysdale, Alastair C. Lewis, Sarah J. Møller, Carole Helfter, Stefan Metzger, Rob Liddard, Eiko Nemitz, Janet F. Barlow, James D. Lee
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Abstract

Road transport NOx emissions in many high-income countries have steadily reduced due to improved exhaust after-treatment technology. However, ambient concentrations of NO2, O3 and PM2.5 continue to exceed World Health Organization guidelines in many cities globally. The megacity of London has taken an international lead in mobility interventions through the use of low-emission zones. Using long-term air pollution flux measurements made from a communications tower, we show that the largest source of NOx emissions in central London has transitioned from road transport to space heating. Observations and supporting consumption/mobility data indicated that natural gas combustion in boilers was responsible for 72 ± 17% of NOx emissions in the measurement footprint (average years 2021–2023). Road transport has dominated air quality thinking on NO2 for many decades. However, in urban environments that are reliant on natural gas, building heating may now be an effective sector to prioritize for further NOx emissions intervention. With system-wide changes in the heat and power sector expected in the coming decades to achieve decarbonisation pledges, we project that very low urban emissions of NOx are achievable. The trajectory will, however, depend on choices made around urban buildings and their associated infrastructure and whether low-carbon fuel combustion or electrification pathways are chosen. We estimate a damage cost penalty of up to £600 M in the U.K. should hydrogen combustion replace natural gas for heating rather than technologies such as heat pumps.

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供暖主导的城市氮氧化物排放的证据
由于废气后处理技术的改进,许多高收入国家的道路运输氮氧化物排放量稳步减少。然而,在全球许多城市,二氧化氮、臭氧和PM2.5的环境浓度继续超过世界卫生组织的指导方针。通过使用低排放区,特大城市伦敦在交通干预方面走在了国际前列。通过对一座通信塔进行的长期空气污染通量测量,我们发现伦敦市中心最大的氮氧化物排放源已经从道路运输转变为空间供暖。观察和支持消耗/移动数据表明,在测量足迹中,锅炉中的天然气燃烧占NOx排放量的72±17%(2021-2023年平均年)。几十年来,道路运输一直主导着对二氧化氮的空气质量思考。然而,在依赖天然气的城市环境中,建筑供暖现在可能是优先考虑进一步干预氮氧化物排放的有效部门。预计在未来几十年,热力和电力行业将发生全系统的变化,以实现脱碳承诺,我们预计,极低的城市氮氧化物排放是可以实现的。然而,发展轨迹将取决于围绕城市建筑及其相关基础设施的选择,以及是否选择低碳燃料燃烧或电气化途径。我们估计,如果氢燃烧代替天然气而不是热泵等技术来供暖,英国的损害成本罚款将高达6亿英镑。
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来源期刊
环境科学与技术
环境科学与技术 环境科学-工程:环境
CiteScore
17.50
自引率
9.60%
发文量
12359
审稿时长
2.8 months
期刊介绍: Environmental Science & Technology (ES&T) is a co-sponsored academic and technical magazine by the Hubei Provincial Environmental Protection Bureau and the Hubei Provincial Academy of Environmental Sciences. Environmental Science & Technology (ES&T) holds the status of Chinese core journals, scientific papers source journals of China, Chinese Science Citation Database source journals, and Chinese Academic Journal Comprehensive Evaluation Database source journals. This publication focuses on the academic field of environmental protection, featuring articles related to environmental protection and technical advancements.
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