城市大气中风致颗粒物组分重悬浮及其与氮氧化物的关系

J. Linda, O. Uhlík, Klaudia Kobolova, J. Pospíšil, T. Apeltauer
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引用次数: 0

摘要

城市大气颗粒物污染是一个持续存在且日益严重的问题。随着电动汽车和低排放热源的逐步发展,重点转向非排气PM排放。风引起的PM重悬浮就是其中之一。这一来源几乎无法采取缓解措施。假设只有粗粒PM (pm10 -2,5)可以被风从地面吹起。通过对长期数据序列的评估,我们可以将PM10浓度分解为PM10-2、5、pmm2、5-1、PM1,并评估它们的行为。这项工作的目的是评估数据,以便识别再悬浮过程,即使是微小的分数,PM1。然后将数据与NOx值进行比较,以确定PM是否来自燃烧过程。在大多数情况下,最初关于NOx和PM1之间存在相关性的假设并未得到证实。结果表明,在某些情况下,粗颗粒物主要与NOx相关。在重悬浮过程中,细颗粒和粗颗粒与NOx的相关性主要取决于一天中的时间段。
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WIND INDUCED RESUSPENSION OF PARTICULATE MATTER FRACTIONS IN URBAN ENVIRONMENT AND THEIR CORRELATION TO NITROGEN OXIDES
Air pollution by particulate matter (PM) in urban environment is an ongoing problem with increasing severity. With the gradual evolution of electromobility and lowemission heat sources, the focus is shifting to non-exhaust PM emissions. Wind induced PM resuspension is one of them. This source is hardly amenable to mitigation measures. It was assumed, that only coarse PM (PM10-2,5) can be lifted from the ground by the wind. By the evaluation of the long-term data series, we can divide the PM10 concentration to its fractions PM10-2,5, PM2,5-1, PM1 and evaluate their behaviour. The aim of the work was to evaluate the data in order to recognize the resuspension process, even with a fine fraction, PM1. The data were then compared with the NOx values to determine if the PM originated from combustion processes. The original assumption of a correlation between NOx and PM1 was not confirmed in most cases. The results show that in some cases coarse PM are dominantly associated with NOx. The correlation of fine and coarse particles with NOx in resuspension process depends primarily on the time period of the day.
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