腔体辅助高分辨率太赫兹光谱仪

IF 2.5 3区 物理与天体物理 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Photonics and Nanostructures-Fundamentals and Applications Pub Date : 2024-01-20 DOI:10.1016/j.photonics.2024.101227
Fabien Simon , Coralie Elmaleh , Jean Decker , Marc Fourmentin , Arnaud Cuisset , Guillaume Ducournau , Jean-François Lampin , Gaël Mouret , Francis Hindle
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引用次数: 0

摘要

利用太赫兹辐射分析气体具有很高的辨别能力,因为在低压下可以观察到很窄的线宽。现有高分辨率仪器的灵敏度受到关键系统组件的可用性和性能的限制。本研究利用两个具有波长尺度物理结构的关键部件来实现高精细太赫兹腔体。对该腔体进行了表征,并将其集成到光谱仪中。实验证明了仪器对痕量和纯气体的灵敏度极限。空腔增强吸收光谱(CEAS)和空腔环降光谱(CRDS)配置均可达到亚ppm检测水平。空腔还被用于测量大气损耗。
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Cavity assisted high-resolution THz spectrometer

The analysis of gases by THz radiation offers a high degree of discrimination due to the narrow linewidths that are observed at low pressure. The sensitivity of existing high-resolution instruments is limited by the availability and performance of critical system components. This study uses two key components with physical structures at the wavelength scale to realise a high finesse THz cavity. The cavity is characterised and incorporated into a spectrometer. Sensitivity limits of the instrument are experimentally demonstrated for trace and pure gases. Both CEAS (Cavity Enhanced Absorption Spectroscopy) and CRDS (Cavity Ring-Down Spectroscopy) configurations are shown to give sub-ppm detection levels. The cavity has also been used to measure the atmospheric losses.

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来源期刊
CiteScore
5.00
自引率
3.70%
发文量
77
审稿时长
62 days
期刊介绍: This journal establishes a dedicated channel for physicists, material scientists, chemists, engineers and computer scientists who are interested in photonics and nanostructures, and especially in research related to photonic crystals, photonic band gaps and metamaterials. The Journal sheds light on the latest developments in this growing field of science that will see the emergence of faster telecommunications and ultimately computers that use light instead of electrons to connect components.
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