14 MeV 中子与镥同位素相互作用的截面及其理论激发函数

Yueli Song, F. Zhou, Yong Li, Xiaopeng Zhang, P. Ji, Xiaojun Sun
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摘要

利用活化技术测量了中子能量为 13.57、14.03、14.62 和 14.86 MeV 时 175Lu(n,p)175Yb、175Lu(n,α)172Tm、176Lu(n,α)173Tm、175Lu(n,2n)174mLu 和 175Lu(n,2n)174gLu 反应的反应截面。这些反应的理论激发函数是通过 Talys-1.95 代码计算得出的。对实验获得的反应截面数据进行了分析,并与文献实验数据、国际原子能机构五大评估核数据图书馆的评估数据以及基于 Talys-1.95 的理论值进行了比较。某些中子能量下的现有数据与部分文献数据以及基于 Talys-1.95 的理论值一致。基于 Talys-1.95 的激发函数理论曲线与现有数据和文献数据的一致性优于 175Lu(n,p)175Yb、175Lu(n,α)172 Tm 和 176Lu(n,α)173Tm 反应的激发函数评估曲线。这项工作将有助于给出聚变堆材料镥的新的评估反应截面数据,提高中子诱导反应截面数据库的质量,推动相关应用研究。
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Cross sections for 14 MeV neutron interaction with lutetium isotopes and their theoretical excitation functions
The reaction cross-sections for the 175Lu(n,p)175Yb, 175Lu(n,α)172Tm, 176Lu(n,α)173Tm, 175Lu(n,2n)174mLu, and 175Lu(n,2n)174gLu reactions at the 13.57, 14.03 14.62 and 14.86 MeV neutron energies were measured by using an activation technique. The theoretical excitation functions of these reactions were calculated by using the Talys-1.95 code. The experimentally obtained reaction cross-section data were analyzed and compared with the literature experimental data, and the evaluated data of five major evaluated nuclear data libraries of IAEA, as well as with the theoretical values based on Talys-1.95. The present data at some neutron energies agree with some of the literature data, and with theoretical values based on Talys-1.95. The consistency of the theoretical curves of excitation functions based on Talys-1.95 with the present and literature data is better than that of the evaluation curves of excitation functions for the 175Lu(n,p)175Yb, 175Lu(n,α)172 Tm, and 176Lu(n,α)173Tm reactions. This work will be helpful to give new evaluated reaction cross-section data on the fusion reactor material lutetium to improve the quality of the neutron-induced reaction cross section data libraries, and advance the related application research.
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