揭开阿拉斯加水和雪地中微塑料污染的面纱

IF 4.3 3区 材料科学 Q1 ENGINEERING, ELECTRICAL & ELECTRONIC ACS Applied Electronic Materials Pub Date : 2024-05-14 DOI:10.1039/D4EW00092G
Subhabrata Dev, Davis Schwarz, Muradur Rashedin, Md Ibnul Hasan, Darya Kholodova, Shane Billings, David L. Barnes, Nicole Misarti, Navid B. Saleh and Srijan Aggarwal
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摘要

虽然微塑料(MPs)在全球海洋环境中普遍存在,并延伸至北极和亚北极地区,但这些地区的陆地水域、饮用水源和娱乐用水中 MPs 的范围和分布情况仍然未知。这项实地研究确定了阿拉斯加三个地理位置(即极北、内陆和中南部)地表水源(包括湖泊、河流和小溪)以及雪中 MPs 的基线。结果(平均值 ± SE)显示,雪地中的 MP 数量最多(681±44 L-1),其次是湖泊(361±76 L-1)、小溪(377±88 L-1)和河流(352±98 L-1)。最小的 MPs(即 89.6±3 µm)也出现在雪地中,其次是湖泊(153.4±13 µm)、河流(267.6±28 µm)和小溪(319.5±25 µm)中的较大 MPs。MPs 的物理形态差异很大。在这些地点,MP 碎片占绝大多数(即近 62-74%),MP 纤维(近 13-21%)、颗粒(近 13-18%)和薄膜(<6%)的数量也相当可观。从地理位置上看,阿拉斯加远北地区的 MP 数量最高(695±58 L-1),而阿拉斯加内陆地区(473±64 L-1)和中南部地区(447±62 L-1)的 MP 数量最低。结果还表明,随着距离最近的海岸线和城镇或社区的距离增加,源水和雪地中 MPs 的出现率也在降低。这些对阿拉斯加陆地水域和降水中 MPs 的基准观测结果表明,即使在开发程度较低的环境中也存在 MP 污染。这可以看作是该地区及其他地区接触多溴联苯及其风险的一个令人担忧的原因。
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Unveiling microplastics pollution in Alaskan waters and snow†

While microplastics (MPs) are globally prevalent in marine environments, extending to the Arctic and sub-Arctic regions, the extent and distribution of MPs in terrestrial waters, drinking water sources, and recreational water in these areas remain unknown. This field study establishes a baseline for MPs in surface water sources, including lakes, rivers, and creeks, as well as in snow across three geo-locations (i.e., Far North, Interior, and Southcentral) in Alaska. Results (mean ± SE) show that the highest MP counts exist in snow (681 ± 45 L−1), followed by lakes (361 ± 76 L−1), creeks (377 ± 88 L−1), and rivers (359 ± 106 L−1). The smallest MPs (i.e., 90.6 ± 4 μm) also happened to have occurred in snow, followed by their larger sizes in lakes (203.9 ± 65 μm), creeks (382.8 ± 136.5 μm), and rivers (455.4 ± 212 μm). The physical morphology of MPs varies widely. MP fragments are predominant (i.e., nearly 62–74%) in these sites, while MP fibers (nearly 13–21%), pellets (nearly 13–18%), and films (<6%) also exist in appreciable quantities. Geolocation-wise, the Far North, where MPs were collected from off-road locations, shows the highest MP counts (695 ± 58 L−1), compared to Interior (473 ± 64 L−1) and Southcentral (447 ± 62 L−1) Alaska. Results also indicate that the occurrence of MPs in the source waters and snow decreases with increasing distance from the nearest coastlines and towns or communities. These baseline observations of MPs in terrestrial waters and precipitation across Alaska indicate MP pollution even in less-explored environments. This can be seen as a cause for concern with regard to MP exposure and risks in the region and beyond.

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