用连续柱法研究北山花岗岩中的铀迁移

IF 1.4 3区 化学 Q4 CHEMISTRY, INORGANIC & NUCLEAR Radiochimica Acta Pub Date : 2024-06-05 DOI:10.1515/ract-2024-0281
Si-yi Gong, Jinguang Zheng, Xin Yang, Yan Ma, Zhenfeng Tong, Tao Chen
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引用次数: 0

摘要

摘要 放射性核素迁移是放射性废物处置库性能和安全评估中的一个重要过程。本研究采用连续柱法研究了铀在北山花岗岩中的迁移,重点关注流速、洗脱液 pH 值和碳酸盐的影响。实验参数用于对迁移过程进行 COMSOL 模拟。研究结果表明,机械分散在花岗岩柱中的铀迁移过程中起着主导作用。值得注意的是,吸附对迁移的影响似乎有限,这可能是由于实验装置中的接触时间很短。这项研究成功展示了 COMSOL 模拟放射性核素迁移的能力,为储存库的性能和安全评估提供了重要启示。
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Migration study of uranium in Beishan granite by the continuous column method
Abstract Radionuclide migration is an essential process in the performance and safety assessments of radioactive waste repository. This study investigates uranium migration in Beishan granite using the continuous column method, focusing on the effects of flow rate, eluent pH, and carbonate. Experimental parameters were used to perform COMSOL simulations of the migration process. The findings reveal that mechanical dispersion plays a predominant role in uranium migration in the granite column. Notably, the impact of adsorption on migration appears to be limited, likely due to the brief contact time in the experimental setup. The study successfully demonstrates the capability of COMSOL in simulating radionuclide migration, offering significant insights for the performance and safety assessments of repository.
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来源期刊
Radiochimica Acta
Radiochimica Acta 化学-核科学技术
CiteScore
2.90
自引率
16.70%
发文量
78
审稿时长
6 months
期刊介绍: Radiochimica Acta publishes manuscripts encompassing chemical aspects of nuclear science and technology.
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