通过低温等离子体混合系统将生物废弃物升级再造为先进碳材料:应用、机理、策略和未来展望

IF 7.1 2区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Waste management Pub Date : 2024-09-04 DOI:10.1016/j.wasman.2024.08.036
Fanghua Li , Gaotingyue Li , Bachirou Guene Lougou , Qiaoqiao Zhou , Boshu Jiang , Yong Shuai
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引用次数: 0

摘要

本综述重点介绍生物废弃物可持续转化为有价值碳质材料的最新进展。本研究总结了通过等离子体混合系统在生物废物衍生碳材料(BCMs)方面取得的重大进展。其中包括基于人工智能的多偶联系统等系统性研究、从经济角度看有前景的合成策略,以及它们在能源、环境和生物医学方面的潜在应用。等离子体改性 BCM 具有新的过渡晶格相,并表现出很高的弹性,同时对等离子体混合系统中 BCM 的制造和形成机制进行了综述。从生物废料中可以设计和制备出独特的二维结构,这种结构具有迷人的物理化学特性,如高比表面积、独特的缺陷位点和优异的导电性。BCMs 的结构为元素掺杂提供了各种活化位点,在电化学领域显示出令人满意的吸附能力和动态性能。近年来,关于将生物废弃物转化为各种应用领域的有价值材料的研究报道很多。合成方法是一个不可或缺的因素,直接影响着生物材料的结构和性能。因此,有必要对低温等离子体混合体系衍生的BCMs的简便合成方法及其形成机理进行综述,这是通过选择合适的合成工艺获得具有理想结构和性能的BCMs的必要条件。先进的碳中性材料可作为催化剂广泛合成,应用于环境修复、能源转换和储存以及生物技术领域。
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Upcycling biowaste into advanced carbon materials via low-temperature plasma hybrid system: applications, mechanisms, strategies and future prospects

This review focuses on the recent advances in the sustainable conversion of biowaste to valuable carbonaceous materials. This study summarizes the significant progress in biowaste-derived carbon materials (BCMs) via a plasma hybrid system. This includes systematic studies like AI-based multi-coupling systems, promising synthesis strategies from an economic point of view, and their potential applications towards energy, environment, and biomedicine. Plasma modified BCM has a new transition lattice phase and exhibits high resilience, while fabrication and formation mechanisms of BCMs are reviewed in plasma hybrid system. A unique 2D structure can be designed and formulated from the biowaste with fascinating physicochemical properties like high surface area, unique defect sites, and excellent conductivity. The structure of BCMs offers various activated sites for element doping and it shows satisfactory adsorption capability, and dynamic performance in the field of electrochemistry. In recent years, many studies have been reported on the biowaste conversion into valuable materials for various applications. Synthesis methods are an indispensable factor that directly affects the structure and properties of BCMs. Therefore, it is imperative to review the facile synthesis methods and the mechanisms behind the formation of BCMs derived from the low-temperature plasma hybrid system, which is the necessity to obtain BCMs having desirable structure and properties by choosing a suitable synthesis process. Advanced carbon–neutral materials could be widely synthesized as catalysts for application in environmental remediation, energy conversion and storage, and biotechnology.

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来源期刊
Waste management
Waste management 环境科学-工程:环境
CiteScore
15.60
自引率
6.20%
发文量
492
审稿时长
39 days
期刊介绍: Waste Management is devoted to the presentation and discussion of information on solid wastes,it covers the entire lifecycle of solid. wastes. Scope: Addresses solid wastes in both industrialized and economically developing countries Covers various types of solid wastes, including: Municipal (e.g., residential, institutional, commercial, light industrial) Agricultural Special (e.g., C and D, healthcare, household hazardous wastes, sewage sludge)
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