活性柱状相中的手性和奇异力学

S J Kole, Gareth P Alexander, Ananyo Maitra, Sriram Ramaswamy
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摘要

手性活性材料在其弹性和粘性响应中都显示出奇异的动力学效应。我们的研究表明,在三维空间中具有二维奇异弹性的最对称介相是手性的、极性的和柱状的,在垂直于柱子的平面上具有二维平移阶,并且它们的相对滑动没有弹性恢复力。我们从模型 H 的手性活动变体推导出其流体力学方程。奇异动力学最显著的预测是两种不同类型的柱状振荡,其频率在零波数时不消失。此外,活动导致了一种屈曲不稳定性,这种不稳定性来自一般的力偶极主动应力,类似于被动材料中的机械赫尔弗里希-胡拉特不稳定性,而手性矩偶极主动应力则通过选择螺旋柱状起伏从根本上改变了这种不稳定性。
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Chirality and odd mechanics in active columnar phases
Chiral active materials display odd dynamical effects in both their elastic and viscous responses. We show that the most symmetric mesophase with two-dimensional odd elasticity in three dimensions is chiral, polar and columnar, with two-dimensional translational order in the plane perpendicular to the columns and no elastic restoring force for their relative sliding. We derive its hydrodynamic equations from those of a chiral active variant of model H. The most striking prediction of the odd dynamics is two distinct types of column oscillation whose frequencies do not vanish at zero wavenumber. In addition, activity leads to a buckling instability coming from the generic force-dipole active stress analogous to the mechanical Helfrich-Hurault instability in passive materials, while the chiral torque-dipole active stress fundamentally modifies the instability by the selection of helical column undulations.
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