Siyuan Zhang, Kaiyong Tang, Li Fu, Mo Zhou, Haijun Fan, Yan Zeng, Zhiyuan Li
{"title":"制备工艺对 NaMgF3:Dy,Eu 的光致发光（OSL）和热致发光（TL）特性的影响研究","authors":"Siyuan Zhang, Kaiyong Tang, Li Fu, Mo Zhou, Haijun Fan, Yan Zeng, Zhiyuan Li","doi":"10.1016/j.radmeas.2024.107297","DOIUrl":null,"url":null,"abstract":"<div><p>OSL fading with storage time after irradiation remains a major obstacle in the development of ideal OSL materials. Dy and Eu co-doped NaMgF<sub>3</sub> are attractive candidates for various rare earth doped matrix materials. In this study, NaMgF<sub>3</sub>:Dy,Eu was synthesized by a solid-state reaction, and the effects of heating temperature, duration, atmosphere, and cooling rate on XRD, TL and OSL properties were studied. A simple, safe, efficient, and time-saving solid-state reaction was identified as a potential method for the preparation of NaMgF<sub>3</sub>:Dy,Eu, which could be optimally prepared by heating at 750 °C for 2 h under nitrogen atmosphere (2 l/min) followed by rapid cooling. The results show that NaMgF<sub>3</sub>:Dy,Eu has a more stable OSL response and an excellent TL glow curve, with only a 0.4% decrease in the OSL signal read after 1 d of dose irradiation compared to that immediately after irradiation, and a high main TL peak at ∼320 °C. It has been indicated the OSL signal in this material seems to be strongly related to the main TL peak. The material has a considerable OSL sensitivity and decay rate than the Luxel Detector. NaMgF<sub>3</sub>:Dy,Eu will have a promising future in the field of OSL dosimetry due to its near tissue equivalence, low OSL fading without preheating, fast OSL decay rate, and predictable and easily reusable dose elimination.</p></div>","PeriodicalId":21055,"journal":{"name":"Radiation Measurements","volume":"178 ","pages":"Article 107297"},"PeriodicalIF":1.6000,"publicationDate":"2024-09-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Study on the effects of preparation processes on OSL and TL properties of NaMgF3:Dy,Eu\",\"authors\":\"Siyuan Zhang, Kaiyong Tang, Li Fu, Mo Zhou, Haijun Fan, Yan Zeng, Zhiyuan Li\",\"doi\":\"10.1016/j.radmeas.2024.107297\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>OSL fading with storage time after irradiation remains a major obstacle in the development of ideal OSL materials. Dy and Eu co-doped NaMgF<sub>3</sub> are attractive candidates for various rare earth doped matrix materials. In this study, NaMgF<sub>3</sub>:Dy,Eu was synthesized by a solid-state reaction, and the effects of heating temperature, duration, atmosphere, and cooling rate on XRD, TL and OSL properties were studied. A simple, safe, efficient, and time-saving solid-state reaction was identified as a potential method for the preparation of NaMgF<sub>3</sub>:Dy,Eu, which could be optimally prepared by heating at 750 °C for 2 h under nitrogen atmosphere (2 l/min) followed by rapid cooling. The results show that NaMgF<sub>3</sub>:Dy,Eu has a more stable OSL response and an excellent TL glow curve, with only a 0.4% decrease in the OSL signal read after 1 d of dose irradiation compared to that immediately after irradiation, and a high main TL peak at ∼320 °C. It has been indicated the OSL signal in this material seems to be strongly related to the main TL peak. The material has a considerable OSL sensitivity and decay rate than the Luxel Detector. NaMgF<sub>3</sub>:Dy,Eu will have a promising future in the field of OSL dosimetry due to its near tissue equivalence, low OSL fading without preheating, fast OSL decay rate, and predictable and easily reusable dose elimination.</p></div>\",\"PeriodicalId\":21055,\"journal\":{\"name\":\"Radiation Measurements\",\"volume\":\"178 \",\"pages\":\"Article 107297\"},\"PeriodicalIF\":1.6000,\"publicationDate\":\"2024-09-10\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Radiation Measurements\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1350448724002452\",\"RegionNum\":3,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"NUCLEAR SCIENCE & TECHNOLOGY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Radiation Measurements","FirstCategoryId":"101","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1350448724002452","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"NUCLEAR SCIENCE & TECHNOLOGY","Score":null,"Total":0}
Study on the effects of preparation processes on OSL and TL properties of NaMgF3:Dy,Eu
OSL fading with storage time after irradiation remains a major obstacle in the development of ideal OSL materials. Dy and Eu co-doped NaMgF3 are attractive candidates for various rare earth doped matrix materials. In this study, NaMgF3:Dy,Eu was synthesized by a solid-state reaction, and the effects of heating temperature, duration, atmosphere, and cooling rate on XRD, TL and OSL properties were studied. A simple, safe, efficient, and time-saving solid-state reaction was identified as a potential method for the preparation of NaMgF3:Dy,Eu, which could be optimally prepared by heating at 750 °C for 2 h under nitrogen atmosphere (2 l/min) followed by rapid cooling. The results show that NaMgF3:Dy,Eu has a more stable OSL response and an excellent TL glow curve, with only a 0.4% decrease in the OSL signal read after 1 d of dose irradiation compared to that immediately after irradiation, and a high main TL peak at ∼320 °C. It has been indicated the OSL signal in this material seems to be strongly related to the main TL peak. The material has a considerable OSL sensitivity and decay rate than the Luxel Detector. NaMgF3:Dy,Eu will have a promising future in the field of OSL dosimetry due to its near tissue equivalence, low OSL fading without preheating, fast OSL decay rate, and predictable and easily reusable dose elimination.
期刊介绍：
The journal seeks to publish papers that present advances in the following areas: spontaneous and stimulated luminescence (including scintillating materials, thermoluminescence, and optically stimulated luminescence); electron spin resonance of natural and synthetic materials; the physics, design and performance of radiation measurements (including computational modelling such as electronic transport simulations); the novel basic aspects of radiation measurement in medical physics. Studies of energy-transfer phenomena, track physics and microdosimetry are also of interest to the journal.
Applications relevant to the journal, particularly where they present novel detection techniques, novel analytical approaches or novel materials, include: personal dosimetry (including dosimetric quantities, active/electronic and passive monitoring techniques for photon, neutron and charged-particle exposures); environmental dosimetry (including methodological advances and predictive models related to radon, but generally excluding local survey results of radon where the main aim is to establish the radiation risk to populations); cosmic and high-energy radiation measurements (including dosimetry, space radiation effects, and single event upsets); dosimetry-based archaeological and Quaternary dating; dosimetry-based approaches to thermochronometry; accident and retrospective dosimetry (including activation detectors), and dosimetry and measurements related to medical applications.
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