{"title":"固有的非线性 Nernst 和 Seebeck 效应","authors":"Harsh Varshney, Amit Agarwal","doi":"arxiv-2409.11108","DOIUrl":null,"url":null,"abstract":"The Nernst and Seebeck effects are crucial for thermoelectric energy\nharvesting. However, the linear anomalous Nernst effect requires magnetic\nmaterials with intrinsically broken time-reversal symmetry. In non-magnetic\nsystems, the dominant transverse thermoelectric response is the nonlinear\nNernst current. Here, we investigate nonlinear Nernst and Seebeck effects to\nreveal intrinsic scattering-free Seebeck and Nernst currents arising from band\ngeometric effects in bipartite antiferromagnets (parity-time-reversal symmetric\nsystems). We show that these contributions, independent of scattering time,\noriginate from the Berry connection polarizability tensor which depends on the\nquantum metric. Using CuMnAs as a model system, we demonstrate the dominance of\nintrinsic nonlinear Seebeck and Nernst currents over other scattering-dependent\ncontributions. Our findings deepen the fundamental understanding of nonlinear\nthermoelectric phenomena and provide the foundation for using them to develop\nmore efficient, next-generation energy harvesting devices.","PeriodicalId":501137,"journal":{"name":"arXiv - PHYS - Mesoscale and Nanoscale Physics","volume":null,"pages":null},"PeriodicalIF":0.0000,"publicationDate":"2024-09-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Intrinsic nonlinear Nernst and Seebeck effect\",\"authors\":\"Harsh Varshney, Amit Agarwal\",\"doi\":\"arxiv-2409.11108\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The Nernst and Seebeck effects are crucial for thermoelectric energy\\nharvesting. However, the linear anomalous Nernst effect requires magnetic\\nmaterials with intrinsically broken time-reversal symmetry. In non-magnetic\\nsystems, the dominant transverse thermoelectric response is the nonlinear\\nNernst current. Here, we investigate nonlinear Nernst and Seebeck effects to\\nreveal intrinsic scattering-free Seebeck and Nernst currents arising from band\\ngeometric effects in bipartite antiferromagnets (parity-time-reversal symmetric\\nsystems). We show that these contributions, independent of scattering time,\\noriginate from the Berry connection polarizability tensor which depends on the\\nquantum metric. Using CuMnAs as a model system, we demonstrate the dominance of\\nintrinsic nonlinear Seebeck and Nernst currents over other scattering-dependent\\ncontributions. Our findings deepen the fundamental understanding of nonlinear\\nthermoelectric phenomena and provide the foundation for using them to develop\\nmore efficient, next-generation energy harvesting devices.\",\"PeriodicalId\":501137,\"journal\":{\"name\":\"arXiv - PHYS - Mesoscale and Nanoscale Physics\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2024-09-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"arXiv - PHYS - Mesoscale and Nanoscale Physics\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/arxiv-2409.11108\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"arXiv - PHYS - Mesoscale and Nanoscale Physics","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/arxiv-2409.11108","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
The Nernst and Seebeck effects are crucial for thermoelectric energy
harvesting. However, the linear anomalous Nernst effect requires magnetic
materials with intrinsically broken time-reversal symmetry. In non-magnetic
systems, the dominant transverse thermoelectric response is the nonlinear
Nernst current. Here, we investigate nonlinear Nernst and Seebeck effects to
reveal intrinsic scattering-free Seebeck and Nernst currents arising from band
geometric effects in bipartite antiferromagnets (parity-time-reversal symmetric
systems). We show that these contributions, independent of scattering time,
originate from the Berry connection polarizability tensor which depends on the
quantum metric. Using CuMnAs as a model system, we demonstrate the dominance of
intrinsic nonlinear Seebeck and Nernst currents over other scattering-dependent
contributions. Our findings deepen the fundamental understanding of nonlinear
thermoelectric phenomena and provide the foundation for using them to develop
more efficient, next-generation energy harvesting devices.