固有的非线性 Nernst 和 Seebeck 效应

Harsh Varshney, Amit Agarwal
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引用次数: 0

摘要

纳斯特效应和塞贝克效应对于热电能量收集至关重要。然而,线性反常的奈恩斯特效应要求磁性材料具有内在的时间反向对称性。在非磁性系统中,主要的横向热电响应是非线性奈恩斯特电流。在这里,我们研究了非线性纳斯特效应和塞贝克效应,揭示了双方反铁磁体(奇偶性-时间反向对称系统)中由带几何效应产生的本征无散射塞贝克电流和纳斯特电流。我们的研究表明,这些贡献与散射时间无关,源于取决于量子度量的贝里连接极化张量。以铜锰砷为模型系统,我们证明了本征非线性塞贝克电流和内斯特电流对其他散射贡献的主导作用。我们的发现加深了对非线性热电现象的基本理解,并为利用它们开发更高效的下一代能量收集器件奠定了基础。
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Intrinsic nonlinear Nernst and Seebeck effect
The Nernst and Seebeck effects are crucial for thermoelectric energy harvesting. However, the linear anomalous Nernst effect requires magnetic materials with intrinsically broken time-reversal symmetry. In non-magnetic systems, the dominant transverse thermoelectric response is the nonlinear Nernst current. Here, we investigate nonlinear Nernst and Seebeck effects to reveal intrinsic scattering-free Seebeck and Nernst currents arising from band geometric effects in bipartite antiferromagnets (parity-time-reversal symmetric systems). We show that these contributions, independent of scattering time, originate from the Berry connection polarizability tensor which depends on the quantum metric. Using CuMnAs as a model system, we demonstrate the dominance of intrinsic nonlinear Seebeck and Nernst currents over other scattering-dependent contributions. Our findings deepen the fundamental understanding of nonlinear thermoelectric phenomena and provide the foundation for using them to develop more efficient, next-generation energy harvesting devices.
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