{"title":"利用轫致辐射优化同位素生产的分析方法","authors":"V.L. Uvarov, A.A. Zakharchenko, N.P. Dikiy, YuV. Lyashko, R.I. Pomatsalyuk","doi":"10.1016/j.apradiso.2024.111547","DOIUrl":null,"url":null,"abstract":"<div><div>Based on analytical description of isotope production by bremsstrahlung (X-ray) radiation, an algorithm is proposed for calculating the optimal dimensions of a cylindrical target of given mass positioned at a given distance from a bremsstrahlung converter to ensure the maximum yield of the isotope product. The expressions are derived for the total activity and its distribution along the target axis. A technique of γ-spectrometric measuring the activity of a thick production target is proposed. The novel approach is validated by the <sup>100</sup>Mo(γ,n)<sup>99</sup>Mo reaction induced in a natural molybdenum target by mass in the range 10–100g with the X-ray photons at an end-point energy of 40 MeV. The analytical predictions are in good agreement with the results of Monte-Carlo simulations and experiment.</div></div>","PeriodicalId":8096,"journal":{"name":"Applied Radiation and Isotopes","volume":"214 ","pages":"Article 111547"},"PeriodicalIF":1.6000,"publicationDate":"2024-10-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"An analytical approach to optimization of isotope production by bremsstrahlung radiation\",\"authors\":\"V.L. Uvarov, A.A. Zakharchenko, N.P. Dikiy, YuV. Lyashko, R.I. Pomatsalyuk\",\"doi\":\"10.1016/j.apradiso.2024.111547\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Based on analytical description of isotope production by bremsstrahlung (X-ray) radiation, an algorithm is proposed for calculating the optimal dimensions of a cylindrical target of given mass positioned at a given distance from a bremsstrahlung converter to ensure the maximum yield of the isotope product. The expressions are derived for the total activity and its distribution along the target axis. A technique of γ-spectrometric measuring the activity of a thick production target is proposed. The novel approach is validated by the <sup>100</sup>Mo(γ,n)<sup>99</sup>Mo reaction induced in a natural molybdenum target by mass in the range 10–100g with the X-ray photons at an end-point energy of 40 MeV. The analytical predictions are in good agreement with the results of Monte-Carlo simulations and experiment.</div></div>\",\"PeriodicalId\":8096,\"journal\":{\"name\":\"Applied Radiation and Isotopes\",\"volume\":\"214 \",\"pages\":\"Article 111547\"},\"PeriodicalIF\":1.6000,\"publicationDate\":\"2024-10-09\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Applied Radiation and Isotopes\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0969804324003750\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, INORGANIC & NUCLEAR\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Applied Radiation and Isotopes","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0969804324003750","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, INORGANIC & NUCLEAR","Score":null,"Total":0}
An analytical approach to optimization of isotope production by bremsstrahlung radiation
Based on analytical description of isotope production by bremsstrahlung (X-ray) radiation, an algorithm is proposed for calculating the optimal dimensions of a cylindrical target of given mass positioned at a given distance from a bremsstrahlung converter to ensure the maximum yield of the isotope product. The expressions are derived for the total activity and its distribution along the target axis. A technique of γ-spectrometric measuring the activity of a thick production target is proposed. The novel approach is validated by the 100Mo(γ,n)99Mo reaction induced in a natural molybdenum target by mass in the range 10–100g with the X-ray photons at an end-point energy of 40 MeV. The analytical predictions are in good agreement with the results of Monte-Carlo simulations and experiment.
期刊介绍：
Applied Radiation and Isotopes provides a high quality medium for the publication of substantial, original and scientific and technological papers on the development and peaceful application of nuclear, radiation and radionuclide techniques in chemistry, physics, biochemistry, biology, medicine, security, engineering and in the earth, planetary and environmental sciences, all including dosimetry. Nuclear techniques are defined in the broadest sense and both experimental and theoretical papers are welcome. They include the development and use of α- and β-particles, X-rays and γ-rays, neutrons and other nuclear particles and radiations from all sources, including radionuclides, synchrotron sources, cyclotrons and reactors and from the natural environment.
The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria.
Papers dealing with radiation processing, i.e., where radiation is used to bring about a biological, chemical or physical change in a material, should be directed to our sister journal Radiation Physics and Chemistry.
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