用于室温下 CO$_{2}$ 传感的 TiO$_{2}$ 装饰 MoS$_{2}$ 纳米复合材料

IF 2.2 Q3 ENGINEERING, ELECTRICAL & ELECTRONIC IEEE Sensors Letters Pub Date : 2024-10-15 DOI:10.1109/LSENS.2024.3480970
Rahul Gond;Prajjwal Shukla;Brajesh Rawat
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引用次数: 0

摘要

由于二氧化碳(CO$_{2}$)对气候变化、窒息风险、农业生产率和人类健康的重大影响,对其进行连续和实时监测已成为一种迫切的需求。用于监测 CO$_{2}$ 的电化学传感器面临着响应时间慢、工作温度高和缺乏选择性等挑战。为了克服这些挑战,我们提出了一种基于 TiO$_{2}$-MoS$_{2}$ 纳米复合材料(NC)的高选择性室温(RT)CO$_{2}$ 检测传感器,该传感器采用丝网印刷方法制造。所制造的传感器在 1000 ppm 时的响应率约为 2.11%,响应/恢复时间接近 102/37s。灵敏度约为 0.0032%/ppm,在 500-5000 ppm 的 CO$_{2}$ 浓度范围内具有出色的响应。尽管非活性 CO$_{2}$ 气体的选择性通常较低,但制造出的传感器却具有很高的选择性,其响应比响应次高的 CO 气体高出约 2.21 倍。这种可扩展的制造方法和实时操作使 TiO$_{2}$-MoS$_{2}$ 传感器成为一种极具成本效益的高性能 CO$_{2}$ 传感产品。
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TiO$_{2}$-Decorated MoS$_{2}$ Nanocomposite for CO$_{2}$ Sensing At Room Temperature
Continuous and real-time monitoring of carbon dioxide (CO $_{2}$ ) has become an urgent demand due to its significant impact on climate change, asphyxiation risks, agricultural productivity, and human health. Electrochemical sensors for CO $_{2}$ monitoring face challenges, such as slow response time, high operating temperature, and lack of selectivity. To overcome these challenges, we propose a highly selective room-temperature (RT) CO $_{2}$ detection sensor based on TiO $_{2}$ -MoS $_{2}$ nanocomposite (NC), which is manufactured using a screen printing methodology. The fabricated sensor achieved a response of approximately 2.11% and response/recovery times of nearly 102/37s at 1000 ppm. The sensitivity is observed to be approximately 0.0032%/ppm with an excellent response for the CO $_{2}$ concentration range of 500–5000 ppm. Despite the typically low selectivity of unreactive CO $_{2}$ gas, the fabricated sensor exhibits high selectivity, with a response of around 2.21× higher than that of the CO gas with the next highest response. The scalable fabrication methodology and RT operation make TiO $_{2}$ -MoS $_{2}$ sensor a highly viable candidate for production through a cost-effective and high performance CO $_{2}$ sensing.
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来源期刊
IEEE Sensors Letters
IEEE Sensors Letters Engineering-Electrical and Electronic Engineering
CiteScore
3.50
自引率
7.10%
发文量
194
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