Elizabeth Asher, Alexandre Baron, Pengfei Yu, Michael Todt, Penny Smale, Ben Liley, Richard Querel, Tetsu Sakai, Isamu Morino, Yoshitaka Jin, Tomohiro Nagai, Osamu Uchino, Emrys Hall, Patrick Cullis, Bryan Johnson, Troy D. Thornberry
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引用次数: 0
摘要
火山和火积云(pyroCB)注入平流层会扰动气溶胶层,并在几个月到几年的时间尺度内产生重要的辐射和化学影响。自2019年以来,我们在南半球(SH)中纬度地区对气溶胶的大小和数量浓度(直径140纳米)、臭氧、水汽和大气状态变量进行了多次现场气球机载测量,使我们能够更好地描述此类事件。我们利用这一记录和重合的激光雷达消光剖面,详细研究了2019年至2022年期间南半球平流层发生的几次中到大规模扰动,包括2020年澳大利亚新年超级暴发(ANYSO)火烧云。还将上海中纬度气溶胶数量浓度、有效半径和表面积的中值垂直剖面与北半球中纬度在基线条件下使用相同有效载荷记录的数据进行了比较。这些数据描述了这一时期 SH 中纬度平流层气溶胶特性的变化,为全球断面气溶胶模型提供了基准。它们揭示了基线条件下和火山羽流中的硫酸盐粒径分布在群落地球系统模型-群落大气气溶胶辐射模型(CESM-CARMA)中得到了相对较好的体现,但还需要对生物质燃烧羽流进行更多的观测,以提高模型模拟热化学气溶胶的技能。原位观测和激光雷达观测之间的比较也突出表明,需要对新鲜和老化生物质燃烧羽流中的气溶胶成分和折射率进行更多观测。
Balloon Baseline Stratospheric Aerosol Profiles (B2SAP)—Perturbations in the Southern Hemisphere, 2019–2022
Volcanic and pyrocumulonimbus (pyroCB) injections into the stratosphere perturb the aerosol layer and can have important radiative and chemical impacts on timescales spanning from months to several years. Repeated in situ balloon-borne measurements of aerosol size and number concentration (>140 nm in diameter), ozone, water vapor, and atmospheric state variables made at midlatitudes in the southern hemisphere (SH) since 2019 enable us to better characterize such events. We use this record and coincident lidar extinction profiles to study several moderate to large stratospheric perturbations in the SH between 2019 and 2022 in detail, including the Australian New Year Super Outbreak (ANYSO) pyroCB in 2020. Median vertical profiles of aerosol number concentration, effective radius, and surface area in SH midlatitudes are also compared with those recorded in Northern Hemisphere midlatitudes under baseline conditions using an identical payload. These data depict the variability in stratospheric aerosol properties in the SH midlatitudes during this period and provide a benchmark for global sectional aerosol models. They reveal that sulfate particle size distributions under baseline conditions and in volcanic plumes are relatively well represented in the Community Earth System Model—Community Aerosol Radiation Model for Atmospheres (CESM-CARMA), but more observations of biomass burning plumes are needed to improve model skill in simulating pyroCB. Comparisons between in situ and lidar observations also highlight a need for more observations of aerosol composition and refractive index in both fresh and aging biomass burning plumes.
期刊介绍:
JGR: Atmospheres publishes articles that advance and improve understanding of atmospheric properties and processes, including the interaction of the atmosphere with other components of the Earth system.