通过 d-T 中子诱导的 natGe(n,x)73Ga 反应形成 73Ga 的截面

IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Radiation Physics and Chemistry Pub Date : 2024-11-12 DOI:10.1016/j.radphyschem.2024.112384
Junhua Luo , Long He , Liang Zhou , Li Jiang
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引用次数: 0

摘要

采用加权平均法,利用四种特征伽马射线测量的截面,研究了在 d-T 中子诱导下通过 natGe(n,x)73Ga 反应形成 73Ga。中子能量和不确定性是通过反应 3H(d,n)4He的 Q 方程结合样品的固角确定的。活化样品的伽马能谱是通过使用高分辨率、高纯度锗探测器(HPGe)的离线技术获得的。分析了核反应 76Ge(n,α)73Zn、73Ge(n,p)73Ga 和 74Ge(n,d∗)73Ga 对残余核 73Ga 的贡献,并确定了反应 73Ge(n,p)73Ga 的横截面,其不确定性很小。利用 TALYS-1.96 软件包对 76Ge(n,α)73Zn、73Ge(n,p)73Ga 和 74Ge(n,d∗)73Ga 反应的截面进行了理论计算。73Ge(n,p)73Ga 核反应的理论计算结果与实验测量结果和数据库提供的评估结果进行了比较。
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Cross-sections for formation of 73Ga through natGe(n, x)73Ga reaction induced by d-T neutrons
The formation of 73Ga through natGe(n,x)73Ga reaction induced by d-T neutrons was investigated using cross-sections measured by four characteristic gamma-rays employing the weighted average method. The neutron energy and uncertainty were determined by the Q equation of reaction 3H(d,n)4He combined with the solid angle of the sample. The gamma spectrum of the activated sample was obtained by an off-line technique using a high-resolution, high-purity germanium detector (HPGe). The contribution of nuclear reactions 76Ge(n,α)73Zn, 73Ge(n,p)73Ga, and 74Ge(n,d∗)73Ga to residual nuclei 73Ga was analyzed and the cross-sections of reaction 73Ge(n,p)73Ga were determined with a small uncertainty. The TALYS-1.96 package was utilized for performing the theoretical calculation of the cross section of 76Ge(n,α)73Zn, 73Ge(n,p)73Ga, and 74Ge(n,d∗)73Ga reactions. The results of the theoretical calculation of nuclear reaction 73Ge(n,p)73Ga were compared with the experimental measurements and the evaluation results provided by the database.
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来源期刊
Radiation Physics and Chemistry
Radiation Physics and Chemistry 化学-核科学技术
CiteScore
5.60
自引率
17.20%
发文量
574
审稿时长
12 weeks
期刊介绍: Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing. The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.
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