交叉蚀刻双曲型超材料使局部电场的宽带和大表面增强成为可能

IF 5.8 3区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nanoscale Pub Date : 2025-01-09 DOI:10.1039/d4nr04039b
Zixian Li, Houjiao Zhang, Zhonghong Shi, Haoyang Li, Guoli He, Shuang Qiu, Zhang-kai Zhou
{"title":"交叉蚀刻双曲型超材料使局部电场的宽带和大表面增强成为可能","authors":"Zixian Li, Houjiao Zhang, Zhonghong Shi, Haoyang Li, Guoli He, Shuang Qiu, Zhang-kai Zhou","doi":"10.1039/d4nr04039b","DOIUrl":null,"url":null,"abstract":"The hyperbolic metamaterials (HMMs) have gained great research efforts, because of their hyperbolic wavevector iso-frequency contour character which leads to great local electric field (EF) enhancements benefiting for boosting optical processes and applications, such as the nonlinear generation, quantum science, biomedical sensing, etc. However, there are mainly three problems of HMMs preventing their practical implementations, which are the difficulty in exciting their resonant modes using free-space incidence, the weak enhancement of surface EF, and the narrow spectral range of EF enhancements. Herein, we propose a kind of new HMMs, which is the cross-etched HMMs (CeHMMs). The CeHMMs can be facially obtained by etching periodic cross-shape arrays in the normal HMMs, and exhibit two resonant high-k modes within the spectral range of 700-1100 nm under the linearly, circularly, or elliptically polarized incident lights from the free space. Also, it is calculated that the CeHMMs can provide large surface EF enhancement in a broadband spectral range (over 500 nm). After integrating the single layered WSe2 onto the top surface, the photoluminescence (PL) enhancements of the CeHMMs and their hot spots based on the emission resonance, are calculated to be 9.72 and 62 times, respectively. With the ability of broadband surface EF enhancement, it is believed the CeHMMs can offer considerable potentials for a variety of nanophotonic applications, including nonlinear optics, integrated optics, and quantum photonics.","PeriodicalId":92,"journal":{"name":"Nanoscale","volume":"20 1","pages":""},"PeriodicalIF":5.8000,"publicationDate":"2025-01-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Broadband and large surface enhancements of local electric field enabled by cross-etched hyperbolic metamaterials\",\"authors\":\"Zixian Li, Houjiao Zhang, Zhonghong Shi, Haoyang Li, Guoli He, Shuang Qiu, Zhang-kai Zhou\",\"doi\":\"10.1039/d4nr04039b\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The hyperbolic metamaterials (HMMs) have gained great research efforts, because of their hyperbolic wavevector iso-frequency contour character which leads to great local electric field (EF) enhancements benefiting for boosting optical processes and applications, such as the nonlinear generation, quantum science, biomedical sensing, etc. However, there are mainly three problems of HMMs preventing their practical implementations, which are the difficulty in exciting their resonant modes using free-space incidence, the weak enhancement of surface EF, and the narrow spectral range of EF enhancements. Herein, we propose a kind of new HMMs, which is the cross-etched HMMs (CeHMMs). The CeHMMs can be facially obtained by etching periodic cross-shape arrays in the normal HMMs, and exhibit two resonant high-k modes within the spectral range of 700-1100 nm under the linearly, circularly, or elliptically polarized incident lights from the free space. Also, it is calculated that the CeHMMs can provide large surface EF enhancement in a broadband spectral range (over 500 nm). After integrating the single layered WSe2 onto the top surface, the photoluminescence (PL) enhancements of the CeHMMs and their hot spots based on the emission resonance, are calculated to be 9.72 and 62 times, respectively. With the ability of broadband surface EF enhancement, it is believed the CeHMMs can offer considerable potentials for a variety of nanophotonic applications, including nonlinear optics, integrated optics, and quantum photonics.\",\"PeriodicalId\":92,\"journal\":{\"name\":\"Nanoscale\",\"volume\":\"20 1\",\"pages\":\"\"},\"PeriodicalIF\":5.8000,\"publicationDate\":\"2025-01-09\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nanoscale\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1039/d4nr04039b\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nanoscale","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1039/d4nr04039b","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

双曲型超材料(HMMs)由于其双曲波矢量等频轮廓特性,使得局部电场(EF)增强,有利于促进光学过程和应用,如非线性生成、量子科学、生物医学传感等。然而,hmm的实际应用主要存在三个问题,即难以利用自由空间入射激发其谐振模式,表面EF增强弱,EF增强的光谱范围窄。在此,我们提出了一种新的hmm,即交叉蚀刻hmm (cross-蚀刻)。通过在普通薄膜上刻蚀周期性的十字形阵列,可以表面得到cehmm,在自由空间的线性、圆或椭圆偏振入射光下,cehmm在700-1100 nm的光谱范围内表现出两种共振高k模式。此外,计算表明cehmm可以在宽带光谱范围(超过500 nm)内提供较大的表面EF增强。将单层WSe2集成到顶表面后,基于发射共振计算cehmm及其热点的光致发光(PL)增强分别为9.72倍和62倍。由于具有宽带表面EF增强的能力,cehmm可以为各种纳米光子应用提供相当大的潜力,包括非线性光学、集成光学和量子光子学。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Broadband and large surface enhancements of local electric field enabled by cross-etched hyperbolic metamaterials
The hyperbolic metamaterials (HMMs) have gained great research efforts, because of their hyperbolic wavevector iso-frequency contour character which leads to great local electric field (EF) enhancements benefiting for boosting optical processes and applications, such as the nonlinear generation, quantum science, biomedical sensing, etc. However, there are mainly three problems of HMMs preventing their practical implementations, which are the difficulty in exciting their resonant modes using free-space incidence, the weak enhancement of surface EF, and the narrow spectral range of EF enhancements. Herein, we propose a kind of new HMMs, which is the cross-etched HMMs (CeHMMs). The CeHMMs can be facially obtained by etching periodic cross-shape arrays in the normal HMMs, and exhibit two resonant high-k modes within the spectral range of 700-1100 nm under the linearly, circularly, or elliptically polarized incident lights from the free space. Also, it is calculated that the CeHMMs can provide large surface EF enhancement in a broadband spectral range (over 500 nm). After integrating the single layered WSe2 onto the top surface, the photoluminescence (PL) enhancements of the CeHMMs and their hot spots based on the emission resonance, are calculated to be 9.72 and 62 times, respectively. With the ability of broadband surface EF enhancement, it is believed the CeHMMs can offer considerable potentials for a variety of nanophotonic applications, including nonlinear optics, integrated optics, and quantum photonics.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Nanoscale
Nanoscale CHEMISTRY, MULTIDISCIPLINARY-NANOSCIENCE & NANOTECHNOLOGY
CiteScore
12.10
自引率
3.00%
发文量
1628
审稿时长
1.6 months
期刊介绍: Nanoscale is a high-impact international journal, publishing high-quality research across nanoscience and nanotechnology. Nanoscale publishes a full mix of research articles on experimental and theoretical work, including reviews, communications, and full papers.Highly interdisciplinary, this journal appeals to scientists, researchers and professionals interested in nanoscience and nanotechnology, quantum materials and quantum technology, including the areas of physics, chemistry, biology, medicine, materials, energy/environment, information technology, detection science, healthcare and drug discovery, and electronics.
期刊最新文献
Intense, self-induced sustainable microwave plasma using carbon nanotubes made from CO2 Synthetic control over lattice strain in trimetallic AuCu-core Pt-shell nanoparticles Significantly enhanced NIR emission of solid-state clusters based on Cu4Pt2 triggered with volatile organic compounds Laser-assisted Thermoelectric Hydrogen Peroxide Biosensor Based on Ag2Se Nanofilms for Sensitive Detection of Bacterial Pathogens NH2-MIL-125(Ti) and its functional nanomaterials – a versatile platform in the photocatalytic arena
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1