大气中的土壤粉尘气溶胶:来源、数量、性质(综述)

Q4 Agricultural and Biological Sciences Biulleten'' Pochvennogo instituta im VV Dokuchaeva Pub Date : 2021-12-25 DOI:10.19047/0136-1694-2021-109-36-95
A. Romanovskaya, I. Savin
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引用次数: 2

摘要

灰尘是大气气溶胶的主要成分,占全球气溶胶负荷的75%。列出了自然和人为来源,以及灰尘研究方法。根据不同的估计,大气中的平均矿物粉尘负荷在20至33 Tg之间,年粉尘排放量为1200至5900 Tg/年。政府间气候变化专门委员会(IPCC)的报告介绍了灰尘的总直接辐射强迫,范围从-0.56到+0.1 W/m2,但对导致这一结果的过程几乎没有科学了解。颗粒大小,包括土壤气溶胶,分为细尘(20μm)。细尘由于太阳辐射的分散而使全球气候降温,而粗尘(大于5μm)通过吸收太阳和热辐射而使气候变暖。然而,对粗尘(20μm以上)的研究仍然很少,关于其含量和排放的数据很少。最近的研究表明,全球模型遗漏的粗尘(17 Tg)对大气加热的平均贡献为0.15 W/m2(0.10至0.24 W/m2),也影响云和降水的全球分布。此外,土壤粉尘的特点是颗粒形状和结构复杂多样,矿物和化学成分不均匀;由于其分散能力和较大的表面积,灰尘与其他类型的气溶胶发生反应,导致颗粒表面形成不同的薄膜或内部混合。所有这些都显著改变了矿尘的光学性质,并使其研究模型的开发变得复杂。
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Soil dust aerosol in the atmosphere: sources, quantities, properties (overview)
Dust is a major component of atmospheric aerosols – 75% of the global aerosol load. Natural and anthropogenic sources are listed, as well as dust research methods. According to different estimates, the average mineral dust load in the atmosphere ranges from 20 to 33 Tg, and the annual dust emission is 1 200–5 900 Tg/year. Reports from the Intergovernmental Panel on Climate Change (IPCC) inform about the total direct radiative forcing of dust ranging from -0.56 to +0.1 W/m2, with little scientific understanding of the processes leading to this result. The particle size, including soil aerosol, is divided into fine (<5 μm), medium (5–10(20) μm) and coarse (>20 μm) dust. Fine dust cools the global climate due to dispersion of solar radiation, while coarse dust (greater than 5 μm) warms the climate by absorbing solar and thermal radiation. However, the coarse dust (above 20 μm) remains poorly investigated, with very little data on its content and emission. Recent studies suggest that coarse dust (17 Tg), missed by the global models, contributes on average 0.15 W/m2 (0.10 to 0.24 W/m2) to atmospheric heating and also affects the global distribution of clouds and precipitation. In addition, soil dust is characterised by a complex and diverse particle shape and structure, heterogeneous mineralogical and chemical composition; due to its dispersion ability and large surface area dust reacts with other types of aerosols, resulting in the formation of different films on the particle surface or internal mixing. All this significantly changes the optical properties of mineral dust and complicates the development of models for its investigation.
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CiteScore
0.90
自引率
0.00%
发文量
15
审稿时长
8 weeks
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