LA103Z镁锂合金表面新型Mg-Al-Co-LDH/MAO复合膜及其主动防腐性能

IF 1.5 4区 材料科学 Q3 MATERIALS SCIENCE, CERAMICS Transactions of the Indian Ceramic Society Pub Date : 2021-10-02 DOI:10.1080/0371750X.2021.2004239
Ju‐mei Zhang, Kai Wang, X. Duan, An‐rong Hou, Jia‐cheng Li, Hui Cai, Zhihu Wang
{"title":"LA103Z镁锂合金表面新型Mg-Al-Co-LDH/MAO复合膜及其主动防腐性能","authors":"Ju‐mei Zhang, Kai Wang, X. Duan, An‐rong Hou, Jia‐cheng Li, Hui Cai, Zhihu Wang","doi":"10.1080/0371750X.2021.2004239","DOIUrl":null,"url":null,"abstract":"In order to further improve the corrosion resistance of the micro-arc oxidization (MAO) film on LA103Z magnesium-lithium alloy, a Mg-Al-Co layered double hydroxide (LDH) film was fabricated on MAO film by an in-situ hydrothermal method. The results showed that with the extension of hydrothermal treatment time, the dense LDH film sealed the micro-pores and cracks in the MAO film successfully. In addition, LDH film treated with a hydrothermal treatment at 90°C for 24 h has the best electrical insulation. The hydrogen evolution rates (mL.cm–2.h−1) of the LDH/MAO composite films rank as LDH/MAO-24 h ≈ LDH/MAO-30 h (0.12) < LDH/MAO-18 h (0.15) < LDH/MAO-12 h (0.16) < MAO (0.25). Meanwhile, the results of potentiodynamic polarization curves showed that the corrosion potential of LDH/MAO-24 h film increased from –1.5349 to −1.388 V, and the corrosion current density decreased by three orders of magnitude. Therefore, the LDH/MAO film has better corrosion resistance than a single MAO film and adds long-term corrosion resistance to the magnesium alloy, which owes to the sealing effect of LDH on inherent defects and trapping effect on corrosion ions. GRAPHICAL ABSTRACT","PeriodicalId":23233,"journal":{"name":"Transactions of the Indian Ceramic Society","volume":"80 1","pages":"251 - 257"},"PeriodicalIF":1.5000,"publicationDate":"2021-10-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"2","resultStr":"{\"title\":\"A Novel Mg-Al-Co LDH/ MAO Composite Films on LA103Z Magnesium-Lithium Alloy and Its Active Anti-corrosion Performance\",\"authors\":\"Ju‐mei Zhang, Kai Wang, X. Duan, An‐rong Hou, Jia‐cheng Li, Hui Cai, Zhihu Wang\",\"doi\":\"10.1080/0371750X.2021.2004239\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"In order to further improve the corrosion resistance of the micro-arc oxidization (MAO) film on LA103Z magnesium-lithium alloy, a Mg-Al-Co layered double hydroxide (LDH) film was fabricated on MAO film by an in-situ hydrothermal method. The results showed that with the extension of hydrothermal treatment time, the dense LDH film sealed the micro-pores and cracks in the MAO film successfully. In addition, LDH film treated with a hydrothermal treatment at 90°C for 24 h has the best electrical insulation. The hydrogen evolution rates (mL.cm–2.h−1) of the LDH/MAO composite films rank as LDH/MAO-24 h ≈ LDH/MAO-30 h (0.12) < LDH/MAO-18 h (0.15) < LDH/MAO-12 h (0.16) < MAO (0.25). Meanwhile, the results of potentiodynamic polarization curves showed that the corrosion potential of LDH/MAO-24 h film increased from –1.5349 to −1.388 V, and the corrosion current density decreased by three orders of magnitude. Therefore, the LDH/MAO film has better corrosion resistance than a single MAO film and adds long-term corrosion resistance to the magnesium alloy, which owes to the sealing effect of LDH on inherent defects and trapping effect on corrosion ions. GRAPHICAL ABSTRACT\",\"PeriodicalId\":23233,\"journal\":{\"name\":\"Transactions of the Indian Ceramic Society\",\"volume\":\"80 1\",\"pages\":\"251 - 257\"},\"PeriodicalIF\":1.5000,\"publicationDate\":\"2021-10-02\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"2\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Transactions of the Indian Ceramic Society\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1080/0371750X.2021.2004239\",\"RegionNum\":4,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"MATERIALS SCIENCE, CERAMICS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Transactions of the Indian Ceramic Society","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1080/0371750X.2021.2004239","RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"MATERIALS SCIENCE, CERAMICS","Score":null,"Total":0}
引用次数: 2

摘要

为了进一步提高LA103Z镁锂合金微弧氧化(MAO)膜的耐蚀性,采用原位水热法在MAO膜上制备了Mg-Al-Co层状双氢氧化物(LDH)膜。结果表明,随着水热处理时间的延长,致密的LDH膜成功地封闭了MAO膜中的微孔和裂纹。此外,经90°C水热处理24小时的LDH膜具有最佳的电绝缘性。LDH/MAO复合膜的析氢速率(mL.cm–2.h−1)为LDH/MAO-24 h≈LDH/MAO-30 h(0.12)<LDH/MAO-18 h(0.15)<LDH/MAO-12 h(0.16)<MAO(0.25),腐蚀电流密度降低了三个数量级。因此,LDH/MAO膜比单一的MAO膜具有更好的耐腐蚀性,并为镁合金增加了长期的耐腐蚀性能,这归因于LDH对固有缺陷的密封作用和对腐蚀离子的捕获作用。图形摘要
本文章由计算机程序翻译,如有差异,请以英文原文为准。
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
A Novel Mg-Al-Co LDH/ MAO Composite Films on LA103Z Magnesium-Lithium Alloy and Its Active Anti-corrosion Performance
In order to further improve the corrosion resistance of the micro-arc oxidization (MAO) film on LA103Z magnesium-lithium alloy, a Mg-Al-Co layered double hydroxide (LDH) film was fabricated on MAO film by an in-situ hydrothermal method. The results showed that with the extension of hydrothermal treatment time, the dense LDH film sealed the micro-pores and cracks in the MAO film successfully. In addition, LDH film treated with a hydrothermal treatment at 90°C for 24 h has the best electrical insulation. The hydrogen evolution rates (mL.cm–2.h−1) of the LDH/MAO composite films rank as LDH/MAO-24 h ≈ LDH/MAO-30 h (0.12) < LDH/MAO-18 h (0.15) < LDH/MAO-12 h (0.16) < MAO (0.25). Meanwhile, the results of potentiodynamic polarization curves showed that the corrosion potential of LDH/MAO-24 h film increased from –1.5349 to −1.388 V, and the corrosion current density decreased by three orders of magnitude. Therefore, the LDH/MAO film has better corrosion resistance than a single MAO film and adds long-term corrosion resistance to the magnesium alloy, which owes to the sealing effect of LDH on inherent defects and trapping effect on corrosion ions. GRAPHICAL ABSTRACT
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Transactions of the Indian Ceramic Society
Transactions of the Indian Ceramic Society 工程技术-材料科学:硅酸盐
CiteScore
2.40
自引率
8.30%
发文量
12
审稿时长
2.3 months
期刊介绍: Transactions of the Indian Ceramic Society is a quarterly Journal devoted to current scientific research, technology and industry-related news on glass and ceramics. The Journal covers subjects such as the chemical, mechanical, optical, electronic and spectroscopic properties of glass and ceramics, and characterization of materials belonging to this family. The Editor invites original research papers, topical reviews, opinions and achievements, as well as industry profiles for publication. The contributions should be accompanied by abstracts, keywords and other details, as outlined in the Instructions for Authors section. News, views and other comments on activities of specific industries and organizations, and also analyses of industrial scenarios are also welcome.
期刊最新文献
Effect of Yb2O3 Addition and Sintering Temperature on the Densification Behavior of Magnesium Aluminate Spinel Powder Perovskite Layer Structure (PLS) Piezoceramics for High Temperature Applications: A Review Effect of Corrosion Inhibitor Pyrovanadate Ions on Microstructure and Corrosion Resistance of MgAl Layered Double Hydroxide Films on LA43M Mg-Li Alloy Doping Mn Induced Modification on the Crystal Structure, Morphology and Optical Properties of Mechanically Activated SrTiO3 Powders Ballistic Resistance of Silicon-Carbide-Based Ceramic and Ultrahigh-Molecular-Weight Polyethylene Composite Armor
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1