辐射诱导烟道气中气溶胶的形成:低剂量的实验

Jyrki M. Mäkelä
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引用次数: 1

摘要

介绍了在潮湿空气中二氧化硫气体辐照诱导气溶胶形成的室内实验。本工作与电子束净化烟气技术中气溶胶粒子的形成过程有关。作为该方法的一个部分过程,水蒸气辐射分解的初级产物将二氧化硫转化为气态硫酸,然后与水蒸气成核形成小的酸滴。这项实验工作是在相对较低的吸收剂量下进行的。气溶胶颗粒的形成与剂量密切相关。在实验中,第一批气溶胶颗粒已经被检测到,吸收剂量为0.1-10毫戈瑞。这些情况下的颗粒尺寸在所谓的超细尺寸范围内(1 - 20nm)。本文介绍了三种实验装置和一些特性结果。
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Irradiation induced aerosol formation in flue gas: Experiments on low doses

Laboratory experiments on irradiation induced aerosol formation from gaseous sulphur dioxide in humid air are presented. This work is connected to the aerosol particle formation process in the electron beam technique for cleaning flue gas. As a partial process of this method primary products of the radiolysis of water vapour convert sulphur dioxide into gaseous sulphuric acid which then nucleates with water vapour forming small acid droplets. This experimental work has been performed on relatively low absorbed doses. Aerosol particle formation is strongly dependent on dose. In the experiments, the first aerosol particles were detected already on absorbed doses of 0.1–10 mGy. The particle size in these cases in the so-called ultrafine size range (1–20 nm). In this article three experimental set-ups with some characteristic results are presented.

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