The effect of surface plasmonic resonances on magneto-plasmonic spherical core-shell nanocomposites

Kinde Yeneayehu, T. Senbeta, B. Mesfin
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Abstract

 In this study, the effect of plasmon resonance on magneto-plasmonic  spherical core-shell nanocomposite enclosed in a dielectric host medium is theoretically investigated by applying electrostatic approximation (esa) and Maxwell-Garnet effective medium theories to obtain magneto-optical parameters such as; effective electric permittivity and magnetic permeability as well as the corresponding extinction cross-sections. Likewise, for a fixed size of QDs (of radius  nm) numerical analysis was performed to determine the plasmonic resonance effect by varying the parameters such as the metal fraction (β) and the dielectrics (εh) of the host medium on the magneto-plasmonic nanostructures (nss). The results depict that graphs of absorption, scattering, and extinction cross-sections as a function of wavelength have two positions of resonance peaks. The first set of peaks are in the ultraviolet (uv) and the second located in visible regions. These peaks originated from the strong coupling between a regular periodic vibrations of surface plasmons of silver (Ag) with the excitonic state of the dielectric/semiconductor at the internal ( ) and external (Ag/host) interfaces. As β increases, the absorption and scattering cross-sections are blue-shifted in the first peak and red shifted the second set of peaks. Similarly, as εh increases or as β decreases, the sets of resonance peaks for extinction cross-section gets enhanced; while keeping one of these parametric quantities fixed at once. The resulting surface plasmon resonance effect might be utilized in a variety of applications that combines both the plasmonic and magnetic core-shell nanostructures ranging from UV to Visible spectral regions.
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表面等离子体共振对磁等离子体球形核壳纳米复合材料的影响
本文应用静电近似(esa)和麦克斯韦-石榴石有效介质理论,从理论上研究了等离子体共振对包裹在介质中的磁等离子体球形核壳纳米复合材料的影响,得到了磁光参数,如;有效介电常数和磁导率以及相应的消光截面。同样,对于固定尺寸的量子点(半径nm),通过改变磁性等离子体纳米结构(nss)上的金属分数(β)和介质介电常数(εh)等参数,进行了数值分析,以确定等离子体共振效应。结果表明,吸收、散射和消光截面随波长的变化曲线有两个共振峰的位置。第一组峰位于紫外线区,第二组峰位于可见光区。这些峰值源于银(Ag)表面等离子体激元的规则周期性振动与介电/半导体在内部(Ag)和外部(Ag/主机)界面的激子态之间的强耦合。随着β的增加,吸收和散射截面在第一峰发生蓝移,在第二峰发生红移。同样地,随着εh的增大或β的减小,消光截面的共振峰组增大;同时保持其中一个参数量不变。由此产生的表面等离子体共振效应可用于从紫外到可见光谱区结合等离子体和磁性核壳纳米结构的各种应用。
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