Characterization of second-order nonlinear optical properties of two-dimensional materials (Conference Presentation)

W. Murray, Yimin Ding, Ethan Kahn, Michael C. Lucking, Y. Yeh, Joshua Noble, X. Ni, H. Terrones, M. Terrones, Zhiwen Liu
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Abstract

We study the second-order nonlinear optical properties of several 2D materials through second harmonic generation (SHG) and sum frequency generation (SFG). SHG signals from 2D transition metal dichalcogenides (TMD) pumped at multiple fundamental wavelengths are measured and compared with theoretical analysis. We also use polarization-resolved second harmonic generation to characterize 2D materials and explore their biological applications. Using a narrow-band femtosecond laser beam and a supercontinuum, we measure the SFG of TMDs to characterize their second-order nonlinear susceptibility over a range of wavelengths.
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二维材料二阶非线性光学性质的表征(会议报告)
通过二次谐波产生(SHG)和和频产生(SFG)研究了几种二维材料的二阶非线性光学性质。对二维过渡金属二硫化物(TMD)在多个基波泵浦下产生的SHG信号进行了测量,并与理论分析进行了比较。我们还使用偏振分辨二次谐波产生来表征二维材料并探索其生物应用。利用窄带飞秒激光束和超连续介质,我们测量了tmd的SFG,以表征其在一定波长范围内的二阶非线性磁化率。
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