BETA-RADIATING RADIONUCLIDES FORMED IN A WATER TARGET OF A COMMERCIAL CYCLOTRON

D. Brinkevich, S. Brinkevich, H. Kiyavitskaya, A. Kiyko
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Abstract

The accumulation of в-emitting radionuclides during irradiation of a liquid target of the Cyclone 18/9 HC commercial cyclotron and the production of radiopharmaceuticals (RP) based on 18F was studied by liquid scintillation spectroscopy. It is shown that with prolonged use of the target in the в-spectra of regenerated water [18O] H2O and ready-made RP [18F] NaF, in addition to the maximum due to tritium, a number of maxima appear in both the low-and high-energy parts of the spectrum. Storage for 3 months leads to a significant transformation of the spectra - the intensity of the low-energy wing of the regenerated water spectrum decreases sharply, the maximum in the 300 channel region disappears, while the intensity of the high-energy wing decreases not so dramatically. It was found that the tritium content in the regenerated water can be reliably estimated only after storage for 3 months.
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在商业回旋加速器的水靶中形成的放射性核素
采用液体闪烁光谱法研究了Cyclone 18/9 HC商用回旋加速器液体靶辐照过程中в-emitting放射性核素的积累及基于18F的放射性药物的生产。结果表明,在再生水[18O] H2O和现成RP [18F] NaF的в-spectra中,随着目标物的长时间使用,除了氚引起的最大值外,在光谱的低能和高能部分都出现了许多最大值。储存3个月后,再生水光谱发生了明显的变化,低能翼的强度急剧下降,300通道区域的最大值消失,而高能翼的强度下降不那么明显。结果表明,再生水中氚的含量需贮存3个月后才能可靠测定。
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