Single molecule spectroscopy: measurements of spectral shifts and fluorescence images

M. Croci, T. Irngartinger, M. Pirotta, V. Palm, T. Plakhotnik, W. Moerner, A. Renn, U. Wild
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Abstract

Spectral shifts of the molecular resonance frequency have been observed since the early days of single molecule spectroscopy (SMS) [4]. We call these effects for concreteness light-induced spectral shifts (LISS) or spontaneous spectral shifts (SSS or S3) to distinguish the two possible reasons for the spectral change. In order to gain a more complete picture of these effects we have undertaken three different approaches.
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单分子光谱学:光谱位移和荧光图像的测量
早在单分子光谱学(SMS)的早期就已经观察到分子共振频率的谱移[4]。我们将这些效应称为混凝土光致光谱位移(LISS)或自发光谱位移(SSS或S3),以区分光谱变化的两种可能原因。为了更全面地了解这些影响,我们采取了三种不同的方法。
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