{"title":"A laminar smoke point-based soot model considering surface growth and soot reactions","authors":"Shahrooz Motaghian, Tarek Beji","doi":"10.1080/13647830.2023.2267526","DOIUrl":null,"url":null,"abstract":"AbstractThis paper proposes a Laminar Smoke Point (LSP)-based soot model, incorporating (as opposed to previously developed LSP-based models) soot surface growth. The latter is indeed believed to be dominant in soot formation. Simple reactions are also introduced to account for the conversion of fuel and oxygen in soot evolution mechanisms. The proposed and a reference LSP-based soot models have been implemented in OpenFOAM-v2006 and assessed against a wide variety of laminar flames (16 flames). A calibration-evaluation procedure is defined in which some flames are involved in the calibration of the constants, and the majority are utilised in an independent evaluation stage. The results show that the newly added features to the LSP-based soot modelling approach allow for a better agreement over a wider range of conditions, e.g. diluted and highly sooty flames. It is shown that although the proposed model is more accurate for buoyant flames, it performs significantly better than the reference model for non-buoyant flames.Keywords: CFDlaminar smoke pointsoot modellingOpenFOAMlaminar diffusion flames Disclosure statementNo potential conflict of interest was reported by the author(s).Additional informationFundingThis work is funded by Ghent University (UGent), Belgium. Project number BOF/STA/201909/008.","PeriodicalId":1,"journal":{"name":"Accounts of Chemical Research","volume":null,"pages":null},"PeriodicalIF":16.4000,"publicationDate":"2023-10-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Accounts of Chemical Research","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.1080/13647830.2023.2267526","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
AbstractThis paper proposes a Laminar Smoke Point (LSP)-based soot model, incorporating (as opposed to previously developed LSP-based models) soot surface growth. The latter is indeed believed to be dominant in soot formation. Simple reactions are also introduced to account for the conversion of fuel and oxygen in soot evolution mechanisms. The proposed and a reference LSP-based soot models have been implemented in OpenFOAM-v2006 and assessed against a wide variety of laminar flames (16 flames). A calibration-evaluation procedure is defined in which some flames are involved in the calibration of the constants, and the majority are utilised in an independent evaluation stage. The results show that the newly added features to the LSP-based soot modelling approach allow for a better agreement over a wider range of conditions, e.g. diluted and highly sooty flames. It is shown that although the proposed model is more accurate for buoyant flames, it performs significantly better than the reference model for non-buoyant flames.Keywords: CFDlaminar smoke pointsoot modellingOpenFOAMlaminar diffusion flames Disclosure statementNo potential conflict of interest was reported by the author(s).Additional informationFundingThis work is funded by Ghent University (UGent), Belgium. Project number BOF/STA/201909/008.
期刊介绍:
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.