Source Attribution of Atmospheric Dust Deposition to Utah Lake

IF 3.1 Q2 WATER RESOURCES Hydrology Pub Date : 2023-11-09 DOI:10.3390/hydrology10110210
Justin T. Telfer, Mitchell M. Brown, Gustavious P. Williams, Kaylee B. Tanner, A. Woodruff Miller, Robert B. Sowby, Theron G. Miller
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Abstract

Atmospheric deposition (AD) is a significant source of nutrient loading to waterbodies around the world. However, the sources and loading rates are poorly understood for major waterbodies and even less understood for local waterbodies. Utah Lake is a eutrophic lake located in central Utah, USA, and has high-nutrient levels. Recent research has identified AD as a significant source of nutrient loading to the lake, though contributions from dust particles make up 10% of total AD. To better understand the dust AD sources, we sampled suspected source locations and collected deposition samples around the lake. We analyzed these samples using Inductively Coupled Plasma (ICP) for 25 metals to characterize their elemental fingerprints. We then compared the lake samples to the source samples to determine likely source locations. We computed spectral angle, coefficient of determination, multi-dimensional scaling, and radar plots to characterize the similarity of the samples. We found that samples from local dust sources were more similar to dust in lake AD samples than samples from distant sources. This suggests that the major source of the dust portion of AD onto Utah Lake is the local empty fields south and west of the lake, and not the farther playa and desert sources as previously suggested. Preliminary data suggest that dust AD is associated with dry, windy conditions and is episodic in nature. We show that AD from dust particles is likely a small portion of the overall AD nutrient loading on Utah Lake, with the dry and precipitation sources contributing most of the load. This case identifies AD sources to Utah Lake and provides an example of data and methods that can be used to assess similarity or perform attribution for dust, soil, and other environmental data. While we use ICP metals, any number of features can be used with these methods if normalized.
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犹他湖大气粉尘的来源归属
大气沉积(AD)是世界各地水体养分负荷的重要来源。然而,对主要水体的来源和加载率了解甚少,对局部水体的了解就更少了。犹他湖是一个富营养化湖泊,位于美国犹他州中部,具有很高的营养水平。最近的研究已经确定AD是湖泊营养负荷的重要来源,尽管来自尘埃颗粒的贡献占AD总量的10%。为了更好地了解沙尘AD的来源,我们对可疑的来源地点进行了采样,并收集了湖泊周围的沉积样本。我们用电感耦合等离子体(ICP)分析了25种金属样品,以表征它们的元素指纹图谱。然后,我们将湖泊样本与源样本进行比较,以确定可能的源位置。我们计算了光谱角、确定系数、多维尺度和雷达图来表征样品的相似性。我们发现来自本地沙尘源的样本比来自远处沙尘源的样本更接近AD湖样本中的沙尘。这表明AD进入犹他湖的粉尘部分的主要来源是湖泊南部和西部的当地空旷地带,而不是先前认为的更远的playa和沙漠来源。初步数据表明,沙尘AD与干燥、多风的条件有关,并且是间歇性的。研究表明,来自尘埃颗粒的AD可能只占犹他湖AD营养负荷的一小部分,干源和降水源贡献了大部分负荷。本案例确定了犹他湖的AD源,并提供了可用于评估相似性或执行粉尘、土壤和其他环境数据归因的数据和方法示例。当我们使用ICP金属时,如果规范化,这些方法可以使用任何数量的特征。
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来源期刊
Hydrology
Hydrology Earth and Planetary Sciences-Earth-Surface Processes
CiteScore
4.90
自引率
21.90%
发文量
192
审稿时长
6 weeks
期刊介绍: Journal of Hydrology publishes original research papers and comprehensive reviews in all the subfields of the hydrological sciences, including water based management and policy issues that impact on economics and society. These comprise, but are not limited to the physical, chemical, biogeochemical, stochastic and systems aspects of surface and groundwater hydrology, hydrometeorology, hydrogeology and hydrogeophysics. Relevant topics incorporating the insights and methodologies of disciplines such as climatology, water resource systems, ecohydrology, geomorphology, soil science, instrumentation and remote sensing, data and information sciences, civil and environmental engineering are within scope. Social science perspectives on hydrological problems such as resource and ecological economics, sociology, psychology and behavioural science, management and policy analysis are also invited. Multi-and interdisciplinary analyses of hydrological problems are within scope. The science published in the Journal of Hydrology is relevant to catchment scales rather than exclusively to a local scale or site. Studies focused on urban hydrological issues are included.
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