Metal Halide Perovskite Light-Emitting Transistor with Tunable Emission Based on Electrically Doped Semiconductor Nanocrystal-Based Microcavities

IF 2.7 Q1 MATERIALS SCIENCE, CERAMICS Ceramics-Switzerland Pub Date : 2023-09-11 DOI:10.3390/ceramics6030116
Francesco Scotognella
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Abstract

Electroluminescence of metal halide perovskites has been widely reported via the fabrication and optimization of light-emitting diodes and light-emitting transistors. Light-emitting transistors are particularly interesting owing to the additional control of the gate voltage on the electroluminescence. In this work, the design of a microcavity, with a defect mode that can be tuned with an applied voltage, integrated with a metal halide light-emitting transistor is shown. The optical properties of the device have been simulated with the transfer matrix method, considering the wavelength-dependent refractive indexes of all the employed materials. The tunability of the microcavity has been obtained via the employment of doped semiconductor nanocrystalline films, which show a tunable plasma frequency and, thus, a tunable refractive index as a function of the applied voltage. Consequently, the tunability of the electroluminescence of the metal halide perovskite light-emitting transistor has been demonstrated.
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基于电掺杂半导体纳米晶微腔的可调谐发射金属卤化物钙钛矿发光晶体管
金属卤化物钙钛矿的电致发光已经通过发光二极管和发光晶体管的制造和优化得到了广泛的报道。由于对电致发光的栅极电压的额外控制,发光晶体管特别有趣。在这项工作中,设计了一个具有缺陷模式的微腔,该缺陷模式可以通过施加电压进行调谐,并与金属卤化物发光晶体管集成。考虑到所采用材料的波长相关折射率,用传递矩阵法模拟了器件的光学特性。微腔的可调性是通过使用掺杂的半导体纳米晶体薄膜获得的,该薄膜显示出可调谐的等离子体频率,因此,可调谐的折射率作为施加电压的函数。因此,证明了金属卤化物钙钛矿发光晶体管电致发光的可调性。
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来源期刊
CiteScore
3.00
自引率
7.10%
发文量
66
审稿时长
10 weeks
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