Magnetic Properties of the Double Perovskite Sr2CrNbO6

IF 1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Journal of Experimental and Theoretical Physics Pub Date : 2023-12-10 DOI:10.1134/s1063776123100096
D. V. Popov, R. G. Batulin, M. A. Cherosov, I. V. Yatsyk, T. I. Chupakhina, Yu. A. Deeva, I. I. Fazlizhanov, R. M. Eremina, T. Maiti
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Abstract

A double perovskite Sr2CrNbO6 powder compound was studied by using X-ray diffraction, AC and DC magnetization, and ESR measurements. Two transitions in antiferromagnetically ordered regimes were observed through magnetization measurements at T = 5 and 2 K and were confirmed by the linear dependence of the magnetization on the applied magnetic field at these temperatures, approximations of the temperature dependence of the ESR linewidth, and AC magnetization. The zero field cooling curve was approximated by Bonner–Fisher law for quasi one dimensional chain with the exchange integral J/kB = 1 K between chromium spins. An approximation of linear part of magnetic susceptibility temperature dependence was performed using Curie–Weiss law. To describe the obtained effective moment μeff = 3.577μB, the presence Cr3+ and Cr4+ ions is estimated at a respective ratio about 0.8 : 0.2.

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双包晶石 Sr2CrNbO6 的磁性能
摘要 通过 X 射线衍射、交流和直流磁化以及 ESR 测量,研究了一种双包晶 Sr2CrNbO6 粉末化合物。在 T = 5 和 2 K 时,通过磁化测量观察到了反铁磁有序态的两个转变,并通过这些温度下磁化对外加磁场的线性依赖性、ESR 线宽的温度依赖性近似值以及交流磁化得到了证实。零磁场冷却曲线近似于准一维链的 Bonner-Fisher 定律,铬自旋之间的交换积分 J/kB = 1 K。使用居里-魏斯定律对磁感应强度温度依赖性的线性部分进行了近似。为了描述所获得的有效磁矩 μeff = 3.577μB,估计 Cr3+ 和 Cr4+ 离子的存在比例分别约为 0.8 : 0.2。
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来源期刊
CiteScore
1.90
自引率
9.10%
发文量
130
审稿时长
3-6 weeks
期刊介绍: Journal of Experimental and Theoretical Physics is one of the most influential physics research journals. Originally based on Russia, this international journal now welcomes manuscripts from all countries in the English or Russian language. It publishes original papers on fundamental theoretical and experimental research in all fields of physics: from solids and liquids to elementary particles and astrophysics.
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