Environmental radioactivity, radiological hazards, and trace elements assessment of nearshore sediment in the Bay of Bengal

IF 4.3 3区 材料科学 Q1 ENGINEERING, ELECTRICAL & ELECTRONIC ACS Applied Electronic Materials Pub Date : 2024-02-01 DOI:10.1016/j.ijsrc.2023.12.002
Manikanda Bharath Karuppasamy , Usha Natesan , Chandrasekaran Seethapathy , Srinivasalu Seshachalam
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Abstract

The current study focuses on the environmental radioactivity and multi-risk assessment of nearshore sediment as a source of marine pollution along the Bay of Bengal. The study examines the distribution of primordial radionuclide concentrations using a thallium-activated sodium iodide (NaI(Tl)) detector-based gamma-ray spectrometer and Potentially Toxic Elements (PTE) through atomic adsorption analysis. The data also were used to characterize ecological threats, radiological risks, and the geospatial distribution of toxic compounds in nearshore sediment as a proxy for marine pollution. The active concentration of primordial radionuclides such as uranium-238 (238U), thorium-232 (232Th), and potassium-40 (40K) was found in the range from ≤ 3 to 68 (11.4), ≤ 9.5 to 142.7 (41.2), and 85.2 to 603.4 (362) Bq/kg, and the results show that the average radioactive concentration of the average radionuclides was less than suggested by the United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR) ranges. Potentially toxic elements iron (Fe), chromium (Cr), nickel (Ni), lead (Pb), and zinc (Zn) were higher in deeper water depths. The current study reveals that mud distribution primarily controls such elements. A decreasing order has been seen as follows by the ecological risk index of individual elements: copper (Cu) > lead (Pb) > nickel (Ni) > chromium (Cr) > zinc (Zn). The significant Pb, Cu, and Zn concentrations indicated high pollution at most stations, possibly resulting from regional and terrestrial sources such as industrial activity, urban drainage, manufacturing, and farming. The migration of contaminated soil from the industrial and transportation sectors may be the source of the increased levels of hazardous elements and naturally occurring radionuclides in the sediment transported into the coastal ecosystems of Bay of Bengal.

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孟加拉湾近岸沉积物的环境放射性、放射性危害和微量元素评估
目前的研究重点是作为孟加拉湾沿岸海洋污染源的近岸沉积物的环境放射性和多重风险评估。本研究使用基于铊活化的碘化钠(NaI(Tl))探测器的伽马射线光谱仪和通过原子吸附分析的潜在有毒元素(PTE)来检测原始放射性核素浓度的分布。这些数据还被用来描述生态威胁、辐射风险和近岸沉积物中有毒化合物的地理空间分布,作为海洋污染的代表。铀-238 (238U)、钍-232 (232Th)和钾-40 (40K)等原始放射性核素的活性浓度在≤3 ~ 68(11.4)、≤9.5 ~ 142.7(41.2)和85.2 ~ 603.4 (362)Bq/kg范围内,结果表明,平均放射性核素的平均放射性浓度低于联合国原子辐射影响科学委员会(UNSCEAR)建议的范围。潜在的有毒元素铁(Fe)、铬(Cr)、镍(Ni)、铅(Pb)和锌(Zn)在水深越深越高。目前的研究表明,泥浆分布主要控制这些因素。各元素生态风险指数的递减顺序为:铜(Cu) >铅(Pb) >镍(Ni) >铬(Cr) >锌(锌)。显著的Pb、Cu和Zn浓度表明大多数站点的污染程度较高,可能是由区域和陆地污染源(如工业活动、城市排水、制造业和农业)造成的。来自工业和运输部门的污染土壤的迁移可能是进入孟加拉湾沿海生态系统的沉积物中有害元素和自然存在的放射性核素水平增加的来源。
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7.20
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4.30%
发文量
567
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