Neutral Tropical African CO2 Exchange Estimated From Aircraft and Satellite Observations

IF 5.4 2区 地球科学 Q1 ENVIRONMENTAL SCIENCES Global Biogeochemical Cycles Pub Date : 2023-12-21 DOI:10.1029/2023GB007804
Benjamin Gaubert, Britton B. Stephens, David F. Baker, Sourish Basu, Michael Bertolacci, Kevin W. Bowman, Rebecca Buchholz, Abhishek Chatterjee, Frédéric Chevallier, Róisín Commane, Noel Cressie, Feng Deng, Nicole Jacobs, Matthew S. Johnson, Shamil S. Maksyutov, Kathryn McKain, Junjie Liu, Zhiqiang Liu, Eric Morgan, Chris O’Dell, Sajeev Philip, Eric Ray, David Schimel, Andrew Schuh, Thomas E. Taylor, Brad Weir, Dave van Wees, Steven C. Wofsy, Andrew Zammit-Mangion, Ning Zeng
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Abstract

Tropical lands play an important role in the global carbon cycle yet their contribution remains uncertain owing to sparse observations. Satellite observations of atmospheric carbon dioxide (CO2) have greatly increased spatial coverage over tropical regions, providing the potential for improved estimates of terrestrial fluxes. Despite this advancement, the spread among satellite-based and in-situ atmospheric CO2 flux inversions over northern tropical Africa (NTA), spanning 0–24°N, remains large. Satellite-based estimates of an annual source of 0.8–1.45 PgC yr−1 challenge our understanding of tropical and global carbon cycling. Here, we compare posterior mole fractions from the suite of inversions participating in the Orbiting Carbon Observatory 2 (OCO-2) Version 10 Model Intercomparison Project (v10 MIP) with independent in-situ airborne observations made over the tropical Atlantic Ocean by the National Aeronautics and Space Administration (NASA) Atmospheric Tomography (ATom) mission during four seasons. We develop emergent constraints on tropical African CO2 fluxes using flux-concentration relationships defined by the model suite. We find an annual flux of 0.14 ± 0.39 PgC yr−1 (mean and standard deviation) for NTA, 2016–2018. The satellite-based flux bias suggests a potential positive concentration bias in OCO-2 B10 and earlier version retrievals over land in NTA during the dry season. Nevertheless, the OCO-2 observations provide improved flux estimates relative to the in situ observing network at other times of year, indicating stronger uptake in NTA during the wet season than the in-situ inversion estimates.

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根据飞机和卫星观测估计的非洲热带二氧化碳中性交换量
热带陆地在全球碳循环中发挥着重要作用,但由于观测稀少,其贡献仍不确定。对大气二氧化碳(CO2)的卫星观测大大增加了对热带地区的空间覆盖,为改进对陆地通量的估计提供了可能。尽管取得了这一进展,但在北纬 0-24 度的热带非洲北部(NTA),基于卫星的大气二氧化碳通量反演和原位大气二氧化碳通量反演之间的差异仍然很大。根据卫星估算,每年的碳源为 0.8-1.45 PgC/yr-1,这对我们了解热带和全球碳循环提出了挑战。在这里,我们将参与轨道碳观测站 2(OCO-2)第 10 版模型相互比较项目(v10 MIP)的一系列反演得出的后验摩尔分数与美国国家航空航天局(NASA)大气层析成像(ATom)任务在热带大西洋上空四个季节进行的独立原位机载观测结果进行了比较。我们利用模型套件定义的通量-浓度关系,对非洲热带地区的二氧化碳通量提出了新的约束条件。我们发现,2016-2018 年 NTA 的年通量为 0.14 ± 0.39 PgC yr-1(平均值和标准偏差)。基于卫星的通量偏差表明,在旱季期间,OCO-2 B10 和早期版本对 NTA 陆地上空的检索可能存在正浓度偏差。尽管如此,相对于一年中其他时间的原位观测网络,OCO-2 观测提供了更好的通量估算,表明与原位反演估算相比,NTA 在雨季的吸收能力更强。
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来源期刊
Global Biogeochemical Cycles
Global Biogeochemical Cycles 环境科学-地球科学综合
CiteScore
8.90
自引率
7.70%
发文量
141
审稿时长
8-16 weeks
期刊介绍: Global Biogeochemical Cycles (GBC) features research on regional to global biogeochemical interactions, as well as more local studies that demonstrate fundamental implications for biogeochemical processing at regional or global scales. Published papers draw on a wide array of methods and knowledge and extend in time from the deep geologic past to recent historical and potential future interactions. This broad scope includes studies that elucidate human activities as interactive components of biogeochemical cycles and physical Earth Systems including climate. Authors are required to make their work accessible to a broad interdisciplinary range of scientists.
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