Thermoelectric Power and Hall Effect in Correlated Metals and Doped Mott–Hubbard Insulators: DMFT Approximation

IF 1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Journal of Experimental and Theoretical Physics Pub Date : 2024-01-26 DOI:10.1134/s1063776123120087
E. Z. Kuchinskii, N. A. Kuleeva, M. V. Sadovskii
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Abstract

We present comparative theoretical investigation of thermoelectric power and Hall effect in the Hubbard model for correlated metal and Mott insulator (considered as prototype cuprate superconductor) for different concentrations of current carriers. Analysis is performed within standard DMFT approximation. For Mott insulator we consider the typical case of partial filling of the lower Hubbard band (hole doping). We calculate the dependence of thermopower on doping level and determine the critical concentration of carriers corresponding to sign change of thermopower. An anomalous dependence of thermopower on temperature is obtained significantly different from linear temperature dependence typical for the usual metals. The role of disorder scattering is analyzed on qualitative level. The comparison with similar studies of the Hall effect shows, that breaking of electron-hole symmetry leads to the appearance of the relatively large interval of band-fillings (close to the half-filling) where thermopower and Hall effects have different signs. We propose a certain scheme allowing to determine the number of carriers from ARPES data and perform semi-quantitative estimate of both thermopower and Hall coefficient using the usual DFT calculations of electronic spectrum.

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相关金属和掺杂莫特-哈伯德绝缘体中的热电动力和霍尔效应:DMFT 近似值
摘要 我们对相关金属和莫特绝缘体(被视为原型铜氧化物超导体)的哈伯德模型中不同载流子浓度下的热电功率和霍尔效应进行了比较理论研究。分析是在标准 DMFT 近似条件下进行的。对于莫特绝缘体,我们考虑了部分填充下哈伯带(空穴掺杂)的典型情况。我们计算了热功率与掺杂水平的关系,并确定了与热功率符号变化相对应的载流子临界浓度。得出的热功率对温度的反常依赖性明显不同于一般金属的典型线性温度依赖性。对无序散射的作用进行了定性分析。与霍尔效应的类似研究进行比较后发现,电子-空穴对称性的破坏导致出现相对较大的带填充区间(接近半填充),在此区间内,热功率和霍尔效应具有不同的符号。我们提出了一种特定的方案,可以通过 ARPES 数据确定载流子的数量,并利用电子频谱的常规 DFT 计算对热功率和霍尔系数进行半定量估算。
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来源期刊
CiteScore
1.90
自引率
9.10%
发文量
130
审稿时长
3-6 weeks
期刊介绍: Journal of Experimental and Theoretical Physics is one of the most influential physics research journals. Originally based on Russia, this international journal now welcomes manuscripts from all countries in the English or Russian language. It publishes original papers on fundamental theoretical and experimental research in all fields of physics: from solids and liquids to elementary particles and astrophysics.
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