Spatially varying optical characteristics in quantum-dot molecules through interdot tunneling

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2024-02-15 DOI:10.1088/1612-202x/ad26ed
R. O. Saleh, M S Mohammed, S. Askar, N. S. A. Darwish, W. R. Kadhum, M. L. Shaghnab, A A Ibrahim, A. Kumar, A. Elawady, A. A. Omran
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Abstract

In this paper, we investigate the spatially dependent absorption characteristics in structurally asymmetric quantum-dot molecules (QDMs), characterized by four energy levels interacting with position-dependent beams and varying system parameters. We explore the effects of detuning, standing wave intensity, and the relative phase of applied fields on the absorption patterns within the medium. A diverse array of patterns emerges, including cross-like structures, ring-like formations, and localized absorption maxima, illustrating the intricate interplay between these parameters and the spatial distribution of absorption features. The introduction of a vortex-shaped control field adds a new dimension to the study, revealing azimuthal dependence and providing a novel perspective for manipulating absorption and gain properties based on the orbital angular momentum of the control field. This work contributes to a comprehensive understanding of the intricate dynamics governing spatially dependent absorption in QDMs, offering valuable insights for controlled manipulation and practical applications in quantum systems.
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量子点分子通过点间隧道实现空间变化的光学特性
在本文中,我们研究了结构不对称量子点分子(QDMs)的空间依赖吸收特性,其特点是四个能级与位置相关的光束相互作用,并且系统参数不断变化。我们探讨了失谐、驻波强度和应用场的相对相位对介质吸收模式的影响。结果发现了多种多样的模式,包括交叉状结构、环状结构和局部吸收最大值,说明了这些参数与吸收特征的空间分布之间错综复杂的相互作用。漩涡状控制场的引入为研究增添了新的维度,揭示了方位角依赖性,并为根据控制场的轨道角动量操纵吸收和增益特性提供了新的视角。这项工作有助于全面了解 QDM 中空间依赖吸收的复杂动力学,为量子系统中的受控操纵和实际应用提供了宝贵的见解。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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