{"title":"Dynamical characteristics of inhomogeneous molecular aggregates","authors":"I. Yu. Ropakova, A. A. Zvyagin","doi":"10.1063/10.0024331","DOIUrl":null,"url":null,"abstract":"The dynamical characteristics of one-dimensional molecular aggregate with the randomness in exciton hopping is considered. We show that the randomness of the distribution of signs of the exciton hopping of the aggregate dramatically changes the dynamical characteristics. In the homogeneous case, the dynamical characteristics of the molecular aggregate manifest narrow lines at edges of the band of Frenkel excitons of the aggregate. On the other hand, we show that the considered randomness yields nonzero contributions to the dynamical characteristics of all excitons of the band.","PeriodicalId":18077,"journal":{"name":"Low Temperature Physics","volume":"17 1","pages":""},"PeriodicalIF":0.6000,"publicationDate":"2024-02-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Low Temperature Physics","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1063/10.0024331","RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q4","JCRName":"PHYSICS, APPLIED","Score":null,"Total":0}
引用次数: 0
Abstract
The dynamical characteristics of one-dimensional molecular aggregate with the randomness in exciton hopping is considered. We show that the randomness of the distribution of signs of the exciton hopping of the aggregate dramatically changes the dynamical characteristics. In the homogeneous case, the dynamical characteristics of the molecular aggregate manifest narrow lines at edges of the band of Frenkel excitons of the aggregate. On the other hand, we show that the considered randomness yields nonzero contributions to the dynamical characteristics of all excitons of the band.
期刊介绍:
Guided by an international editorial board, Low Temperature Physics (LTP) communicates the results of important experimental and theoretical studies conducted at low temperatures. LTP offers key work in such areas as superconductivity, magnetism, lattice dynamics, quantum liquids and crystals, cryocrystals, low-dimensional and disordered systems, electronic properties of normal metals and alloys, and critical phenomena. The journal publishes original articles on new experimental and theoretical results as well as review articles, brief communications, memoirs, and biographies.
Low Temperature Physics, a translation of the copyrighted Journal FIZIKA NIZKIKH TEMPERATUR, is a monthly journal containing English reports of current research in the field of the low temperature physics. The translation began with the 1975 issues. One volume is published annually beginning with the January issues.