Local scale air quality impacts in the Los Angeles Basin from increased port activity during 2021 supply chain disruptions†

IF 2.8 Q3 ENVIRONMENTAL SCIENCES Environmental science: atmospheres Pub Date : 2024-01-31 DOI:10.1039/D3EA00166K
T. Nash Skipper, Jennifer Kaiser, M. Talat Odman, Sina Hasheminassab and Armistead G. Russell
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Abstract

Increased throughput and container ship backlogs at the ports of Los Angeles and Long Beach due to supply chain disruptions related to the COVID-19 pandemic caused a significant increase in the number of ships near the California coast, leading to concerns about increased air pollution exposure of nearby communities. We use a combination of satellite-based observations from TROPOMI and ground-based observations from routine surface monitoring sites with chemical transport model results to analyze the changes in NO2 and PM2.5 in the Los Angeles Basin during a period in 2021 when the number of ships was at its peak. Using simulations to account for meteorological effects, changes are apportioned to emissions and meteorology. The largest emission-related changes in column NO2 occurred immediately east of the ports where emission-related NO2 increased by 28% compared to the baseline (2018–2019 average). In Central Los Angeles, emission reductions led to a 10% decrease in NO2 during the same period. Emission-related PM2.5 increased by 0.7 μg m−3 on average with a maximum increase of 4.5 μg m−3 in the eastern part of Basin. The emission/meteorology attribution method presented here provides a novel approach to quantify emission-influenced changes in air quality that are consistent with observations and suggests that both NO2 and PM2.5 were elevated in parts of the Los Angeles area during a period of increased port activity.

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2021 年供应链中断期间港口活动增加对洛杉矶盆地当地空气质量的影响†。
由于 COVID-19 大流行造成的供应链中断,洛杉矶港和长滩港的吞吐量增加,集装箱船积压,导致加利福尼亚海岸附近的船只数量大幅增加,从而引发了对附近社区空气污染暴露增加的担忧。我们将 TROPOMI 的卫星观测数据和常规地表监测点的地面观测数据与化学传输模型结果相结合,分析了 2021 年船舶数量达到峰值期间洛杉矶盆地二氧化氮和 PM2.5 的变化情况。通过模拟来考虑气象影响,将变化归因于排放和气象。与排放相关的二氧化氮柱变化最大,紧邻港口东部,与排放相关的二氧化氮与基线(2018-2019 年平均值)相比增加了 28%。在洛杉矶中部,排放减少导致同期二氧化氮下降了 10%。与排放相关的 PM2.5 平均增加了 0.7 μg m-3,盆地东部的最大增幅为 4.5 μg m-3。本文介绍的排放/气象归因方法提供了一种新方法,用于量化受排放影响的空气质量变化,该方法与观测结果一致,并表明在港口活动增加期间,洛杉矶部分地区的二氧化氮和 PM2.5 均有所升高。
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