Germanium Fabry-Perot nanoresonators investigated by cathodoluminescence spectroscopy

IF 17.7 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2024-03-18 DOI:10.1051/jeos/2024012
Paolo Biagioni
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Abstract

We report on the experimental investigation, by means of spatially-resolved cathodoluminescence spectroscopy, of rectangular all-dielectric Ge nanoantennas sustaining Fabry-Perot resonances. The combination of spatial and spectral resolution allows us to directly image the standing-wave pattern of the local density of optical states inside the nanoantennas, which is the fingerprint of the resonant Purcell contribution to the overall emission enhancement previously reported in the literature for the same structures. Our results confirm that the emission properties of Ge nanostructures can be effectively tuned by engineering the local density of optical states and that cathodoluminescence provides valuable information to experimentally address such modulation in their emission properties.
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利用阴极发光光谱研究锗法布里-珀罗纳米谐振器
我们报告了通过空间分辨阴极荧光光谱法对维持法布里-珀罗共振的矩形全介质 Ge 纳米天线进行的实验研究。空间分辨率和光谱分辨率的结合使我们能够直接对纳米天线内部光学态局部密度的驻波模式进行成像,这就是之前文献中报道的相同结构的共振普赛尔对整体发射增强的贡献。我们的研究结果证实,Ge 纳米结构的发射特性可以通过对局部光态密度的工程设计进行有效调整,而阴极荧光则为实验解决发射特性的这种调制问题提供了宝贵的信息。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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