Preparation of Single Atom Catalysts for High Sensitive Gas Sensing

IF 18.2 1区 材料科学 Q1 CHEMISTRY, PHYSICAL ACS Energy Letters Pub Date : 2024-03-12 DOI:10.1088/2631-7990/ad3316
Xinxin He, Ping Guo, Xunyang An, Yuyang Li, Jiatai Chen, Xinyu Zhang, Lifeng Wang, Mingjin Dai, Chaoliang Tan, Jia Zhang
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Abstract

Single atom catalysts (SACs) have received enormous attention in the field of catalysis in the last decade due to their maximum atom utilization as well as unique physical and chemical properties. For the semiconductor-based electrical gas sensor, the core is the catalysis process of target gas molecules on the sensitive materials. In this scenario, the SACs would be used for highly sensitive and selective gas sensing, however, only some of bubbles come to the surface. To realize its practical applications, the preparation strategies for SACs are reviewed systematically. The aggregation and low loading of SACs are still the main challenges. Following, the interaction between the SACs and the target gas molecules and its supports is unrevealed to explain the improvement of sensing performances. Furthermore, the typical applications of SACs in the different gases sensing are highlighted, revealing its superiority of high sensitivity and selectivity. Finally, the challenges and future perspectives on the SACs based gas sensing are presented.
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制备用于高灵敏度气体传感的单原子催化剂
近十年来,单原子催化剂(SAC)因其最大程度的原子利用率以及独特的物理和化学特性而在催化领域受到极大关注。对于基于半导体的电子气体传感器来说,其核心是目标气体分子在敏感材料上的催化过程。在这种情况下,SAC 可用于高灵敏度和高选择性的气体传感,但只有部分气泡浮出表面。为了实现其实际应用,本文对 SACs 的制备策略进行了系统综述。SACs 的聚集和低负载仍是主要挑战。其次,SACs 与目标气体分子及其支撑物之间的相互作用尚未被揭示,因此无法解释如何提高传感性能。此外,还重点介绍了 SACs 在不同气体传感中的典型应用,揭示了其高灵敏度和高选择性的优越性。最后,介绍了基于 SACs 的气体传感所面临的挑战和未来展望。
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来源期刊
ACS Energy Letters
ACS Energy Letters Energy-Renewable Energy, Sustainability and the Environment
CiteScore
31.20
自引率
5.00%
发文量
469
审稿时长
1 months
期刊介绍: ACS Energy Letters is a monthly journal that publishes papers reporting new scientific advances in energy research. The journal focuses on topics that are of interest to scientists working in the fundamental and applied sciences. Rapid publication is a central criterion for acceptance, and the journal is known for its quick publication times, with an average of 4-6 weeks from submission to web publication in As Soon As Publishable format. ACS Energy Letters is ranked as the number one journal in the Web of Science Electrochemistry category. It also ranks within the top 10 journals for Physical Chemistry, Energy & Fuels, and Nanoscience & Nanotechnology. The journal offers several types of articles, including Letters, Energy Express, Perspectives, Reviews, Editorials, Viewpoints and Energy Focus. Additionally, authors have the option to submit videos that summarize or support the information presented in a Perspective or Review article, which can be highlighted on the journal's website. ACS Energy Letters is abstracted and indexed in Chemical Abstracts Service/SciFinder, EBSCO-summon, PubMed, Web of Science, Scopus and Portico.
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