Flexible field-effect transistors with high-quality and uniform single-layer graphene for high mobility

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2024-03-07 DOI:10.1088/1361-6641/ad3111
Hyunjin Park, Jimin Kwon, Jihyung Seo, Kiho Kim, Yun Ho Kim, Sungjune Jung
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Abstract

In this work, a fully flexible graphene field-effect transistor with high carrier mobility is reported. Patterned high-quality and uniform single-layer graphene films are successfully realized by combining the selective growth on a patterned copper foil and the direct transfer method to minimize degradation factors. The selectively grown single-layer graphene is directly transferred to the target substrate through the deposition of poly-para-xylylene (Parylene) C. The quality of the graphene films is confirmed by Raman spectroscopy. The analysis reveals that the use of Parylene C as the substrate, gate dielectric, and encapsulation layer has the advantage of reducing the scattering by the optical phonons and charge puddles. The estimated residual carrier density is 1.72 × 1011 cm−2, and the intrinsic hole and electron carrier mobilities are found to be as high as 10260 and 10010 cm2·V−1·s−1, respectively. This study can pave the way for the development and mass production of high-performance and fully flexible graphene electronics.
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采用高质量均匀单层石墨烯的柔性场效应晶体管,可实现高迁移率
本研究报告了一种具有高载流子迁移率的全柔性石墨烯场效应晶体管。通过在图案化铜箔上选择性生长和直接转移法相结合,成功实现了图案化的高质量均匀单层石墨烯薄膜,从而最大限度地减少了降解因素。通过沉积聚对二甲苯(Parylene)C,选择性生长的单层石墨烯被直接转移到目标基底上。分析表明,使用聚对二甲苯 C 作为衬底、栅介质和封装层具有减少光声子散射和电荷坑的优点。估计的剩余载流子密度为 1.72 × 1011 cm-2,本征空穴和电子载流子迁移率分别高达 10260 和 10010 cm2-V-1-s-1。这项研究可为开发和量产高性能、完全柔性的石墨烯电子器件铺平道路。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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