Investigation on the thermal maturity, organic matter sources and depositional environment of lacustrine source rocks in the Dongying Formation of the Bozhong Sag, Bohai Bay Basin, China

IF 1.4 4区 地球科学 Q3 GEOSCIENCES, MULTIDISCIPLINARY Geological Journal Pub Date : 2024-03-27 DOI:10.1002/gj.4956
Guoxiong Li, Chenglin Liu, Zhangxing Chen, Rizwan Sarwar Awan, Feilong Wang, Guangyuan Wang, Hong Yang, Xiaoxiang Zeng, Yuping Wu, Dehao Feng, Taozheng Yang, Zhen-gang Ding
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Abstract

The unclear understanding of the source rock characteristics for the Paleogene Dongying Formation in the Bozhong Sag leads to the lack of cognition in oil and gas exploration. This research systematically evaluated the discrepancy in geochemical characteristics of source rock intervals in the Dongying Formation based on detailed analysis using Rock-Eval pyrolysis, total organic carbon (TOC), vitrinite reflectance (Ro), maceral components, stable carbon isotopes and biomarker parameters. It discusses the organic matter sources, depositional environment, thermal maturity and hydrocarbon generation potential in the source rock intervals of the Dongying Formation. The organic matter abundance in the third member (E3d3) and lower sub-member of the second member (E3d2L) of the Dongying Formation is higher, with an average TOC of 2.08% and 1.03%, respectively, indicating that these source rock intervals could have good and excellent quality. The source rocks of the Dongying Formation predominately contain exinite maceral group and type II1 and II2 kerogen. The thermal evolution is mainly in the low-mature and mature stages. The organic matter sources in the Dongying Formation are mainly dominated by mixed origin (the carbon isotope reversal of aromatics also provides a potential explanation). However, the values of 1,2,5−/1,3,6-trimethylnaphthalene, (1,2,5,6 + 1,2,3,5)-tetramethylnaphthalene/tetramethylnaphthalenes, methyldibenzofuran/methylphenanthrene (MDBF/MP) and dibenzofuran/phenanthrene (DBF/PHEN) parameters in the E3d3 and some samples in E3d2L decipher relatively smaller values than other source rock intervals, proving the enhancement of the contribution of lower organisms. Moreover, the terrestrial input in the bottom-up deposition process of the Dongying Formation gradually increases. The depositional environment reveals the Dongying Formation source rocks mainly developed freshwater sulphur-poor lacustrine facies and shallow lake-fluvial delta facies in an open clay-rich sedimentary environment with poor water column stratification, belonging to the typical weak oxidation–reduction depositional conditions. The comprehensive geochemical evaluation concludes that the favourable supply of lower organisms and stable clay-rich depositional environment in the E3d3 interval of the Dongying Formation are potential explanations for the formation of lacustrine source rocks with high organic matter abundance, intermediate thermal evolution and excellent hydrocarbon generation potential, providing a good foundation for the exploration and development prospects of hydrocarbons.

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中国渤海湾盆地渤中相东营地层湖底源岩的热成熟度、有机质来源及沉积环境研究
由于对渤中海沟古近系东营地层的源岩特征认识不清,导致在油气勘探中缺乏认知。本研究利用Rock-Eval热裂解、总有机碳(TOC)、玻璃光泽反射率(Ro)、巨矿物组分、稳定碳同位素和生物标志物参数进行详细分析,系统评价了东营地层源岩间地球化学特征的差异。报告讨论了东营地层源岩层段的有机质来源、沉积环境、热成熟度和碳氢化合物生成潜力。东营地层第三系(E3d3)和第二系下亚系(E3d2L)的有机质丰度较高,平均总有机碳含量分别为2.08%和1.03%,表明这些源岩层段可能具有良好和优异的质量。东营地层的源岩主要含有外生巨岩组和 II1、II2 型角质。热演化主要处于低成熟和成熟阶段。东营地层的有机质来源主要以混合来源为主(芳烃的碳同位素反转也是一种可能的解释)。然而,1,2,5-/1,3,6-三甲基萘、(1,2,5,6 + 1,2,3,5)-四甲基萘/四甲基萘E3d3 中的甲基二苯并呋喃/甲基菲(MDBF/MP)和二苯并呋喃/菲(DBF/PHEN)参数以及 E3d2L 中的部分样品的参数值相对于其他源岩区间较小,证明低等生物的贡献增加。此外,在东营地层自下而上的沉积过程中,陆相输入量逐渐增加。沉积环境显示,东营地层源岩主要发育淡水贫硫湖相和浅湖-河流三角洲相,处于水柱分层较差的开阔富粘土沉积环境中,属于典型的弱氧化-还原沉积条件。综合地球化学评价认为,东营地层 E3d3 区间有利的低等生物补给和稳定的富粘土沉积环境是形成有机质丰度高、热演化中等、生烃潜力大的湖泊源岩的潜在原因,为油气勘探开发前景提供了良好的基础。
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来源期刊
Geological Journal
Geological Journal 地学-地球科学综合
CiteScore
4.20
自引率
11.10%
发文量
269
审稿时长
3 months
期刊介绍: In recent years there has been a growth of specialist journals within geological sciences. Nevertheless, there is an important role for a journal of an interdisciplinary kind. Traditionally, GEOLOGICAL JOURNAL has been such a journal and continues in its aim of promoting interest in all branches of the Geological Sciences, through publication of original research papers and review articles. The journal publishes Special Issues with a common theme or regional coverage e.g. Chinese Dinosaurs; Tectonics of the Eastern Mediterranean, Triassic basins of the Central and North Atlantic Borderlands). These are extensively cited. The Journal has a particular interest in publishing papers on regional case studies from any global locality which have conclusions of general interest. Such papers may emphasize aspects across the full spectrum of geological sciences.
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