Self-characterization of irradiation facility using synthetic multi-element standard for determination of k0-factors of seven radionuclides of interest

Phonesavanh Lathdavong, Ho Manh Dung, Hồ Văn Doanh, T. Q. Thiện, Trương Trường Sơn
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Abstract

In this study, the k0 factors of 7 short and medium-lived radionuclides (i.e. 66Cu, 52V, 38Cl, 134mCs, 128I, 140La and 56Mn) were experimentally determined at the Dalat nuclear research reactor (DNRR). The synthetic multi-element standard (SMELS) samples were irradiated at Channel 7-1 installed at the DNRR. SMELS Type III contains Au and Zr, thus also allowing the self-characterization of the irradiation facility (i.e. the direct determination of f and a with only this material). The k0 factors of 7 short and medium-lived radionuclides obtained in this work are a good agreement with the reference k0 factors. The ratio values between the experimental and reference k0 values were 66Cu of 1.004, 52V of 1.004, 38Cl of 0.961 and 0.976 (1642.7 keV and 2167.4keV, respectively), 134mCs of 0.831, 128I of 1.022, 140La of 0.936, 0.955 and 0.955 (328.8 keV, 487.0 keV and 1596.2keV, respectively), 56Mn of 0.985 and 0.973 (846.8 keV and 1810.7keV, respectively). The radionuclides range of uncertainty values were lower than 7%. The present result indicates that the k0 factors can be determined by using synthetic multi-element standards (SMELS).
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利用合成多元素标准测定七种相关放射性核素的 k0 因子,实现辐照设施的自我特征描述
本研究在达叻核研究反应堆(DNRR)对 7 种中短寿命放射性核素(即 66Cu、52V、38Cl、134mCs、128I、140La 和 56Mn)的 k0 因子进行了实验测定。合成多元素标准(SMELS)样品在达叻核研究反应堆安装的 7-1 频道进行辐照。SMELS III 型含有金和锆,因此也允许对辐照设施进行自我表征(即只用这种材料直接测定 f 和 a)。这项工作获得的 7 种中短寿命放射性核素的 k0 因子与参考 k0 因子非常吻合。实验值与参考 k0 值的比值分别为:66Cu 为 1.004、52V 为 1.004、38Cl 为 0.961 和 0.976(分别为 1642.7 keV 和 2167.4 keV)、134mCs 为 0.831、128I 为 1.831(分别为 1642.7 keV 和 2167.4 keV)。831, 128I of 1.022, 140La of 0.936, 0.955 and 0.955 (分别为 328.8 keV, 487.0 keV and 1596.2 keV), 56Mn of 0.985 and 0.973 (分别为 846.8 keV and 1810.7 keV)。放射性核素的不确定值范围均低于 7%。本结果表明,使用合成多元素标准(SMELS)可以确定 k0 因子。
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